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Anum Zafar, Karolina Matuszek, Douglas R. MacFarlane, Xinyi Zhang. Recent progress and future perspectives of ionic liquid-based carbon dioxide capture and conversion. Green Energy&Environment, 2025, 10(6): 1097-1129. doi: 10.1016/j.gee.2024.10.002
Citation: Anum Zafar, Karolina Matuszek, Douglas R. MacFarlane, Xinyi Zhang. Recent progress and future perspectives of ionic liquid-based carbon dioxide capture and conversion. Green Energy&Environment, 2025, 10(6): 1097-1129. doi: 10.1016/j.gee.2024.10.002
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Recent progress and future perspectives of ionic liquid-based carbon dioxide capture and conversion

doi: 10.1016/j.gee.2024.10.002

  • a. Hubei Key Laboratory of Micro-Nanoelectronic Materials and Devices, School of Microelectronics, Hubei University, Wuhan, 430062, China;

  • b. Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory, Foshan, 528216, China;

  • c. School of Chemistry, Monash University, Victoria, 3800, Australia

Funds:

This work was supported by the National Natural Science Foundation of China (21972027) and the Foshan Xianhu Laboratory (41220103, 41210501, XHD2021-001, XHD2022-001, 492305, 472303).

  • Received date 17 June 2024, Accepted date 08 October 2024, RevRecd date 10 September 2024, Available online 01 July 2025, Publish date 15 October 2024,
    Abstract
  • Carbon dioxide accounts for about 80 percent of greenhouse emissions and the increasing CO2 emission has been identified as a critical environmental issue. On the other hand, CO2 is a potentially renewable resource of a single carbon molecule, and new technologies to utilize CO2 in producing net-zero fuels and chemicals are of global interest. Great efforts have been made in the development of new materials and processes for CO2 capture and utilization (CCU). Among them, ionic liquids (ILs) have attracted much attention due to their unique characteristics such as high CO2 solubility, high ionic conductivity, negligible volatility, non-flammability, wide electrochemical window, and high thermal stability, as well as good solvation ability. This review summarizes the most recent efforts devoted to IL-based absorption, catalysts, and CO2 capture and utilization processes. We discuss the factors that affect the interaction between ILs and CO2, impacting on the viscosity and CO2 solubility and preview the coupling of CO2 capture with electrochemical conversion of CO2. Finally, we provide an overview on the advantages and disadvantages of the IL-based process for practical applications.

     

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