Turn off MathJax
Article Contents
Article Navigation >  Green Energy&Environment  > 2024  > Accepted Manuscript
Jianran Ren, Zhiliang Zhu, Yanling Qiu, Fei Yu, Tao Zhou, Jie Ma, Jianfu Zhao. Simultaneous Adsorption-Reduction Boosted by In-situ Magnetic Field. Green Energy&Environment. doi: 10.1016/j.gee.2024.04.006
Citation: Jianran Ren, Zhiliang Zhu, Yanling Qiu, Fei Yu, Tao Zhou, Jie Ma, Jianfu Zhao. Simultaneous Adsorption-Reduction Boosted by In-situ Magnetic Field. Green Energy&Environment. doi: 10.1016/j.gee.2024.04.006
shu

Simultaneous Adsorption-Reduction Boosted by In-situ Magnetic Field

doi: 10.1016/j.gee.2024.04.006

  • 1 Research Center for Environmental Functional Materials, State Key Laboratory of Pollution Control and Resource Reuse, College of Environmental Science and Engineering, Tongji University, Shanghai, 200092, China.;

  • 2 School of Civil Engineering, Kashi University, Kashi. 844000, China;

  • 3 College of Marine Ecology and Environment, Shanghai Ocean University, Shanghai, 201306, China

Funds:

This research is supported by The National Natural Science Foundation of China (52170087, 22276137). We are also thankful to the anonymous reviewers for their valuable comments to improve this manuscript.

More Information
  • Author Bio:

    Jianran Ren,E-mail:renjianran@tongji.edu.cn;Yanling Qiu,E-mail:ylqiu@tongji.edu.cn;Fei Yu,E-mail:fyu@vip.163.com;Tao Zhou,E-mail:1410421@tongji.edu.cn;Jianfu Zhao,E-mail:zhaojianfu@tongji.edu.cn

  • Received date 04 December 2023, Accepted date 10 April 2024, RevRecd date 31 March 2024, Available online 24 April 2024
    Abstract
  • The mainstream silver recovery has problems such as resource waste, weak silver selectivity, and complicated operation. Here, self-propelled magnetic enhanced capture hydrogel (magnetic NbFeB/MXene/GO, MNMGH) was prepared by self-crosslinking encapsulation method. MNMGH achieved high selectivity (Kd=23.31 mL/g) in the acidic range, and exhibited ultrahigh silver recovery capacity (1604.8 mg/g), which greatly improved by 66 % with the assistance of in-situ magnetic field. The recovered silver crystals could be directly physically exfoliated, without acid/base additions. The selective sieving effect of adsorption, MNMGH preferentially adsorbed Ag(I), and then selectively reduced to Ag(0), realizing dual-selective recovery. The in-situ magnetic field enhanced selective adsorption by enhancing mass transfer, reactivity of oxygen- containing functional groups. Furthermore, density function theory simulations demonstrated that the in-situ magnetic field could lower the silver reduction reaction energy barrier to enhance the selective reduction. Three-drive synergy system (reduction drive, adsorption drive and magnetic drive) achieved ultrahigh silver recovery performance. This study pioneered an in-situ magnetic field assisted enhancement strategy for dual-selective (adsorption/reduction) recovery of precious metal silver, which provided new idea for low-carbon recovery of noble metal from industrial waste liquids.

     

    • FullText(HTML)
  • loading
    • References(51)
  • [1]
    A. Oluwalowo, N. Nguyen, S. Zhang, J. G. Park, R. Liang, Carbon 146(2019)224-231.
    [2]
    S. P. Deshmukh, S. Patil, S. Mullani, S. Delekar, Mater. Sci. Eng., C 97(2019)954-965.
    [3]
    L. Yang, Y. Tu, H. Li, W. Zhan, H. Hu, Y. Wei, C. Chen, K. Liu, P. Shao, M. Li, Angew. Chem. Int. Ed. 62(2023) e202308702.
    [4]
    L. Yang, Z. Gao, T. Liu, M. Huang, G. Liu, Y. Feng, P. Shao, X. Luo, Environ. Sci. Technol. 57(2023)4591-4597.
    [5]
    Y. Zhao, Y. Ding, W. Li, C. Liu, Y. Li, Z. Zhao, Y. Shan, F. Li, L. Sun, F. Li, Nat. Commun. 14(2023)4491.
    [6]
    K. Z. Elwakeel, A. S. Al-Bogami, E. Guibal, Chem. Eng. J. 403(2021)126265.
    [7]
    K. Krishna, Int. J. Phy. Sci. 4(2009)893-905.
    [8]
    M. B. Mooiman, K. C. Sole, N. Dinham, Met. Sustain.:GC, CP (2016)109-132.
    [9]
    H.-Y. Kang, J. M. Schoenung, Resour. Conserv. Recycl. 45(2005)368-400.
    [10]
    B. Drif, Y. Taha, R. Hakkou, M. Benzaazoua, Miner. Eng. 170(2021)107060.
    [11]
    C. Lei, B. Yan, T. Chen, X.-L. Wang, X.-M. Xiao, J. Clean. Prod. 181(2018)408-415.
    [12]
    F. Pooley, Nature 296(1982)642-643.
    [13]
    Y. Du, X. Tong, X. Xie, W. Zhang, H. Yang, Q. Song, Minerals 11(2021)586.
    [14]
    A. DąBrowski, Z. Hubicki, P. Podkościelny, E. Robens, Chemosphere 56(2004)91-106.
    [15]
    F. Almomani, R. Bhosale, M. Khraisheh, T. Almomani, Appl. Surf. Sci. 506(2020)144924.
    [16]
    C. Wang, X. Hu, M.-L. Chen, Y.-H. Wu, J. Hazard. Mater. 119(2005)245-249.
    [17]
    V. Gurusamy, R. Krishnamoorthy, B. Gopal, V. Veeraravagan, Inorg. Nano-Met. Chem. 47(2017)761-767.
    [18]
    J. Yu. Precious Metals Separation and Refining Technology. Chemical Industry Press, Beijing. 2006.
    [19]
    L. Xiao, Y. Wang, Y. Yu, G. Fu, P. Han, Z. Sun, S. Ye, J. Clean. Prod. 187(2018)708-716.
    [20]
    Z. Yao, P. Shao, D. Fang, J. Shao, D. Li, L. Liu, Y. Huang, Z. Yu, L. Yang, K. Yu, Chem. Eng. J. 427(2022)131470.
    [21]
    P. Shao, D. Liang, L. Yang, H. Shi, Z. Xiong, L. Ding, X. Yin, K. Zhang, X. Luo, J. Hazard. Mater. 387(2020)121676.
    [22]
    P. Shao, Z. Chang, M. Li, X. Lu, W. Jiang, K. Zhang, X. Luo, L. Yang, Nat. Commun. 14(2023)1365.
    [23]
    Y. Huang, W. Zhao, X. Zhang, H. Peng, Y. Gong, Chem. Eng. J. 375(2019)121935.
    [24]
    L. Xie, Z. Yu, S. M. Islam, K. Shi, Y. Cheng, M. Yuan, J. Zhao, G. Sun, H. Li, S. Ma, Adv. Funct. Mater. 28(2018)1800502.
    [25]
    M. Yuan, H. Yao, L. Xie, X. Liu, H. Wang, S. M. Islam, K. Shi, Z. Yu, G. Sun, H. Li, J. Am. Chem. Soc. 142(2019)1574-1583.
    [26]
    T. Shang, Z. Lin, C. Qi, X. Liu, P. Li, Y. Tao, Z. Wu, D. Li, P. Simon, Q. H. Yang, Adv. Funct. Mater. 29(2019)1903960.
    [27]
    H. Li, P. Liu, Y. Liang, J. Xiao, G. Yang, Nanoscale 4(2012)5082-5091.
    [28]
    F. Wu, T. Zhao, Y. Yao, T. Jiang, B. Wang, M. Wang, Chemosphere 238(2020)124638.
    [29]
    L. Yang, L. Xie, M. Chu, H. Wang, M. Yuan, Z. Yu, C. Wang, H. Yao, S. M. Islam, K. Shi, Angew. Chem. 134(2022) e202112511.
    [30]
    L. Ma, Q. Wang, S. M. Islam, Y. Liu, S. Ma, M. G. Kanatzidis, J. Am. Chem. Soc. 138(2016)2858-2866.
    [31]
    Z. Qin, H. Deng, R. Huang, S. Tong, Chem. Eng. J. 428(2022)132493.
    [32]
    L. Zhang, Z. Zeng, D.-W. Wang, Y. Zuo, J. Chen, X. Yan, Cell Rep. Phys. Sci. 2(2021)100455.
    [33]
    Y. Zhang, C. Liang, J. Wu, H. Liu, B. Zhang, Z. Jiang, S. Li, P. Xu, ACS Appl. Energy Mater. 3(2020)10303-10316.
    [34]
    K. Shen, X. Xu, Y. Tang, Nano Energy 92(2022)106703.
    [35]
    L. Zhang, Z. Zeng, D.-W. Wang, Y. Zuo, J. Chen, X. Yan, Cell Rep. Phys. Sci.(2021)100455.
    [36]
    S.-S. Chen, C.-Y. Cheng, C.-W. Li, P.-H. Chai, Y.-M. Chang, J. Hazard. Mater. 142(2007)362-367.
    [37]
    F. Liu, S. You, Z. Wang, Y. Liu, ACS ES&T Eng. 1(2021)1342-1350.
    [38]
    Z. Liu, M. Frasconi, J. Lei, Z. J. Brown, Z. Zhu, D. Cao, J. Iehl, G. Liu, A. C. Fahrenbach, Y. Y. Botros, Nat. Commun. 4(2013)1-9.
    [39]
    L. Ling, X. Y. Huang, W. X. Zhang, Adv. Mater. 30(2018)1705703.
    [40]
    R. Yang, Q. Zhao, B. Liu, J. Mater. Sci.:Mater. Electron. 31(2020)5054-5067.
    [41]
    M. Padilla Villavicencio, A. Escobedo Morales, M. Ruiz Peralta, M. Sánchez-Cantú, L. Rojas Blanco, E. Chigo Anota, J. H. Camacho García, F. Tzompantzi, Catal Lett. 150(2020)2385-2399.
    [42]
    R. Shvab, E. Hryha, L. Nyborg, Powder Metall. 60(2017)42-48.
    [43]
    B. R. Chrcanovic, A. R. Pedrosa, M. D. Martins, Mater. Res. 15(2012)372-382.
    [44]
    P. K. Kalambate, A. Sinha, Y. Li, Y. Shen, Y. Huang, Microchim. Acta 187(2020)1-12.
    [45]
    W. Vallejo, A. Rueda, C. Diaz-Uribe, C. Grande, P. Quintana, R. Soc. Open Sci. 6(2019)181824.
    [46]
    Y. Wan, X. Chen, G. Xiong, R. Guo, H. Luo, Materials Express 4(2014)429-434(426).
    [47]
    G. Li, W. Zhu, C. Zhang, S. Zhang, L. Liu, L. Zhu, W. Zhao, Bioresour. Technol. 206(2016)16-22.
    [48]
    J. Ferreira De Brito, L. De Oliveira Ferreira, M. C. Ragozoni Pereira, J. Paulo Da Silva, T. C. Ramalho, Water, Air, Soil Pollut. 223(2012)3545-3551.
    [49]
    L. Yang, F. Jia, S. Song, Sep. Purif. Technol. 186(2017)63-69.
    [50]
    L. Wu, L. Zeng, X. Jiang, J. Am. Chem. Soc. 137(2015)10052-10055.
    [51]
    X. Ren, T. Wu, Y. Sun, Y. Li, G. Xian, X. Liu, C. Shen, J. Gracia, H.-J. Gao, H. Yang, Nat. Commun. 12(2021)1-12.
    • Relative Articles
    • Supplements(0)
    • Cited By
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Get Citation
    PDF
    XML

    Article Metrics

    Article views (54) PDF downloads(5) Cited by()
    Proportional views

    Publish With GEE

    Contact

    • Email：gee@ipe.ac.cn
    • Tel：010-82627075
    • Address：North 2nd street, Zhongguancun, Haidian District, Beijing, China

    Links

    京ICP备10002620号-1京公网安备 11010802039050号

    Supported by: Beijing Renhe Information Technology Co. Ltd    

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return