Volume 9 Issue 11
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Ping Liu, Kaixing Cai, Keliang Wang, Tianxiang Zhao, Duan-Jian Tao. Highly defective HKUST-1 with excellent stability and SO2 uptake: The hydrophobic armor effect of functionalized ionic liquids. Green Energy&Environment, 2024, 9(11): 1711-1723. doi: 10.1016/j.gee.2023.10.003
Citation: Ping Liu, Kaixing Cai, Keliang Wang, Tianxiang Zhao, Duan-Jian Tao. Highly defective HKUST-1 with excellent stability and SO2 uptake: The hydrophobic armor effect of functionalized ionic liquids. Green Energy&Environment, 2024, 9(11): 1711-1723. doi: 10.1016/j.gee.2023.10.003
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Highly defective HKUST-1 with excellent stability and SO2 uptake: The hydrophobic armor effect of functionalized ionic liquids

doi: 10.1016/j.gee.2023.10.003

  • a. Key Laboratory of Green Chemical and Clean Energy Technology, School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, 550025, China;

  • b. Engineering Research Center of Efficient Utilization for Industrial Waste, Guizhou University, Guiyang, Guizhou, 550025, China;

  • c. School of Chemistry and Materials Engineering, Liupanshui Normal University, Liupanshui, 553004, China;

  • d. College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang, 330022, China

Funds:

This work was supported by the National Natural Science Foundation of China (nos.22168012 and 22208070), the Key Laboratory of Carbon-based Energy Molecular Chemical Utilization Technology in Guizhou Province (no.2023008), and the Guizhou Province Outstanding Young Scientific and Technological Talents Program (no.YQK2023007). We also would like to thank the researchers in the Shiyanjia Lab (www.shiyanjia.com) for their helping with TEM analysis and language editing service.

  • Received date 10 May 2023, Accepted date 07 October 2023, RevRecd date 26 September 2023, Publish date 11 October 2023,
    Abstract
  • Water stability is one of the most important factors restricting the practical application of metal organic frameworks (MOFs). In this work, we fabricate a highly defective HKUST-1 framework with a mixed valence of CuI/CuII by mechanical ball milling method. This defective HKUST-1 is embellished by functionalized ionic liquids as hydrophobic armor, making the hybrid HIL1@HKUST-1 exhibits outstanding water stability, remarkable SO2 adsorption (up to 5.71 mmol g-1), and record-breaking selectivity (1070 for SO2/CO2 and 31,515 for SO2/N2) at 25 ℃ and 0.1 bar, even in wet conditions.

     

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