Volume 9 Issue 8
Aug.  2024
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Article Navigation >  Green Energy&Environment  > 2024  >  9(8): 1290-1305
Changjian Yuan, Xianglei Liu, Xinrui Wang, Chao Song, Hangbin Zheng, Cheng Tian, Ke Gao, Nan Sun, Zhixing Jiang, Yimin Xuan, Yulong Ding. Rapid and stable calcium-looping solar thermochemical energy storage via co-doping binary sulfate and Al–Mn–Fe oxides. Green Energy&Environment, 2024, 9(8): 1290-1305. doi: 10.1016/j.gee.2023.02.009
Citation: Changjian Yuan, Xianglei Liu, Xinrui Wang, Chao Song, Hangbin Zheng, Cheng Tian, Ke Gao, Nan Sun, Zhixing Jiang, Yimin Xuan, Yulong Ding. Rapid and stable calcium-looping solar thermochemical energy storage via co-doping binary sulfate and Al–Mn–Fe oxides. Green Energy&Environment, 2024, 9(8): 1290-1305. doi: 10.1016/j.gee.2023.02.009
shu

Rapid and stable calcium-looping solar thermochemical energy storage via co-doping binary sulfate and Al–Mn–Fe oxides

doi: 10.1016/j.gee.2023.02.009

  • a. School of Energy and Power Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, China;

  • b. Key Laboratory of Thermal Management and Energy Utilization of Aviation Vehicles, Ministry of Industry and Information Technology, Nanjing, 210016, China;

  • c. Birmingham Centre for Energy Storage, School of Chemical Engineering, University of Birmingham, Birmingham, B15 2TT, UK

Funds:

This work was supported by the National Natural Science Foundation of China [No. 51820105010 and 51888103]. XL also wants to thank the support from Jiangsu Province (No. BK20202008, BE2022024, BE2022602, BK20220001, BK20220009, and BK20220077).

  • Received date 25 November 2022, Accepted date 23 February 2023, RevRecd date 22 February 2023, Publish date 02 March 2023,
    Abstract
  • Solar thermochemical energy storage based on calcium looping (CaL) process is a promising technology for next-generation concentrated solar power (CSP) systems. However, conventional calcium carbonate (CaCO3) pellets suffer from slow reaction kinetics, poor stability, and low solar absorptance. Here, we successfully realized high power density and highly stable solar thermochemical energy storage/release by synergistically accelerating energy storage/release via binary sulfate and promoting cycle stability, mechanical strength, and solar absorptance via Al–Mn–Fe oxides. The energy storage density of proposed CaCO3 pellets is still as high as 1455 kJ kg-1 with only a slight decay rate of 4.91% over 100 cycles, which is higher than that of state-of-the-art pellets in the literature, in stark contrast to 69.9% of pure CaCO3 pellets over 35 cycles. Compared with pure CaCO3, the energy storage power density or decomposition rate is improved by 120% due to lower activation energy and promotion of Ca2+ diffusion by binary sulfate. The energy release or carbonation rate rises by 10% because of high O2- transport ability of molten binary sulfate. Benefiting from fast energy storage/release rate and high solar absorptance, thermochemical energy storage efficiency is enhanced by more than 50% under direct solar irradiation. This work paves the way for application of direct solar thermochemical energy storage techniques via achieving fast energy storage/release rate, high energy density, good cyclic stability, and high solar absorptance simultaneously.

     

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