Volume 9 Issue 7
Jul.  2024
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Article Navigation >  Green Energy&Environment  > 2024  >  9(7): 1151-1158
Shunfa Zhou, Yuxuan Liu, Jing Li, Zhao Liu, Jiawei Shi, Liyuan Fan, Weiwei Cai. Surface-neutralization engineered NiCo-LDH/phosphate hetero-sheets toward robust oxygen evolution reaction. Green Energy&Environment, 2024, 9(7): 1151-1158. doi: 10.1016/j.gee.2022.12.003
Citation: Shunfa Zhou, Yuxuan Liu, Jing Li, Zhao Liu, Jiawei Shi, Liyuan Fan, Weiwei Cai. Surface-neutralization engineered NiCo-LDH/phosphate hetero-sheets toward robust oxygen evolution reaction. Green Energy&Environment, 2024, 9(7): 1151-1158. doi: 10.1016/j.gee.2022.12.003
shu

Surface-neutralization engineered NiCo-LDH/phosphate hetero-sheets toward robust oxygen evolution reaction

doi: 10.1016/j.gee.2022.12.003

  • a. Sustainable Energy Laboratory, Faculty of Materials Science and Chemistry, China University of Geosciences, Wuhan, 430074, China;

  • b. College of Science and Engineering, James Cook University, 1 James Cook Drive, Townsville, QLD, 4811, Australia

Funds:

We are grateful for financial support from the National Natural Science Foundation of China (21875224 and 22179121), Knowledge Innovation Program of Wuhan-Basic Research (2022010801010202) and Research Fund Program of Guangdong Provincial Key Laboratory of Fuel Cell Technology (FC202201). The authors would like to thank SCI-GO (www.sci-go.com) for the contact angle analysis.

  • Received date 30 October 2022, Accepted date 09 December 2022, RevRecd date 24 November 2022, Publish date 31 July 2024,
    Abstract
  • Developing highly active oxygen evolution reaction (OER) electrocatalysts with robust durability is essential in producing high-purity hydrogen through water electrolysis. Layered double hydroxide (LDH) based catalysts have demonstrated efficient catalytic performance toward the relatively sluggish OER. By considering the promotion effect of phosphate (Pi) on proton transfer, herein, a facile phosphate acid (PA) surface-neutralization strategy is developed to in-situ construct NiCo-LDH/NiCoPi hetero-sheets toward OER catalysis. OER activity of NiCo-LDH is significantly boosted due to the proton promotion effect and the electronic modulation effect of NiCoPi. As a result, the facilely prepared NiCo-LDH/NiCoPi catalyst displays superior OER catalytic activity with a low overpotential of 300 mV to deliver 100 mA cm-2 OER and a Tafel slope of 73 mV dec-1. Furthermore, no visible activity decay is detected after a 200-h continuous OER operation. The present work, therefore, provides a promising strategy to exploit robust OER electrocatalysts for commercial water electrolysers.

     

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