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Ao Ma, Hengjiang Cong, Hexiang Deng. Multivariate MOF for optimizing atmospheric water harvesting. Green Energy&Environment, 2022, 7(4): 575-577. doi: 10.1016/j.gee.2022.02.004
Citation: Ao Ma, Hengjiang Cong, Hexiang Deng. Multivariate MOF for optimizing atmospheric water harvesting. Green Energy&Environment, 2022, 7(4): 575-577. doi: 10.1016/j.gee.2022.02.004
shu

Multivariate MOF for optimizing atmospheric water harvesting

doi: 10.1016/j.gee.2022.02.004

  • a College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, 430072, China;

  • b Hubei Yangtze Memory Laboratories, Wuhan, 430205, China;

  • c Engineering Research Center of Organosilicon Compounds and Materials-Ministry of Education, College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, 430072, China;

  • d Key Laboratory of Biomedical Polymers-Ministry of Education, College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, 430072, China

Funds:

This work was supported by the National Natural Science Foundation of China (Grant Nos. 21471118, 21971199, 22025106, 51202127, 91545205, and 91622103), National Key Research and Development Project of China (2018YFA0704000), Natural Science Foundation of Hubei Province (2016CFB382), and Fundamental Research Funds for the Central Universities (2042017kf0227, 2042019kf0205).

  • Received date 24 December 2021, Accepted date 08 February 2022, RevRecd date 04 February 2022, Publish date 15 February 2022,
    Abstract
  • Atmospheric water harvesting offers a powerful and promising solution to address the problem of global freshwater scarcity. In the past decade, significant progress has been achieved in utilizing hydrolytically stable metal-organic frameworks as recyclable water-sorbent materials under low relative humidity, especially in those arid areas. Recently, Yaghi's group has employed a combined crystallographic and theoretical technique to decipher the water filling mechanism in MOF-303, where the polar organic linkers rather than the inorganic units of MOF are demonstrated as the key factor. Hence, the hydrophilic strength of the water-binding pocket in MOFs can be optimized through the approach of multivariate modulations, resulting in enhanced water harvesting properties.

     

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