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Ting-Hao Xu, Sin Liou, Fan-Lin Hou, Yuan-Yao Li. Potassium-doped hydrated manganese dioxide nanowires-carbon nanotube on graphene for high performance rechargeable zinc-ion battery. Green Energy&Environment. doi: 10.1016/j.gee.2021.10.006
Citation: Ting-Hao Xu, Sin Liou, Fan-Lin Hou, Yuan-Yao Li. Potassium-doped hydrated manganese dioxide nanowires-carbon nanotube on graphene for high performance rechargeable zinc-ion battery. Green Energy&Environment. doi: 10.1016/j.gee.2021.10.006
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Potassium-doped hydrated manganese dioxide nanowires-carbon nanotube on graphene for high performance rechargeable zinc-ion battery

doi: 10.1016/j.gee.2021.10.006

  • a Department of Chemical Engineering, National Chung Cheng University, Chia-Yi, 62102, Taiwan;

  • b Advanced Institute of Manufacturing with High-Tech Innovations, National Chung Cheng University, Chia-Yi, 62102, Taiwan

Funds:

The authors would like to thank the Ministry of Science and Technology, Taiwan, for supporting this research under grant MOST 109-2221-E-194-015- and the Advanced Institute of Manufacturing with High-tech Innovations (AIM-HI) from The Featured Areas Research Centre Program within the framework of the Higher Education Sprout Project by the Ministry of Education (MOE) in Taiwan.

  • Received date 22 September 2021, Accepted date 28 October 2021, RevRecd date 19 October 2021, Available online 02 December 2021
    Abstract
  • Aqueous rechargeable Zn-ion battery (ARZIB) is a great candidate for the next generation battery due to its high safety, low cost, and relatively high capacity. Here, we develop hydrated and potassium-doped manganese dioxide (MO) nanowires mixed with carbon nanotubes (CNT) on graphene substrates (hydrated KMO-CNT/graphene) for ARZIB. A simple polyol process (poly(ethyl glycol), KMnO4, CNTs, and graphene) is conducted to form the hydrated KMO-CNT/graphene. MnO2 nanowires with diameters of 15–25 nm have a high specific capacity with a short diffusion path. The intercalated K ions and hydrates in the layered MnO2 nanowires remain the MO structure during the charge and discharge process, while carbon nanomaterials (CNTs and graphene) enhance the conductivity of the materials. As a result, the hydrated KMOCNT/graphene demonstrates a good ARZIB performance. A high capacity of 359.8 mAh g-1 at 0.1 A g-1 can be achieved while, at a high current density of 3.0 A g-1, the capacity of 129 mAh g-1 can be obtained with 77% retention after 1000 cycles.

     

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