Volume 7 Issue 3
Jun.  2022
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Article Navigation >  Green Energy&Environment  > 2022  >  7(3): 372-393
Zexu Chi, Jingyun Zhao, Yi Zhang, Han Yu, Hongbing Yu. The fabrication of atomically thin-MoS2 based photoanodes for photoelectrochemical energy conversion and environment remediation: A review. Green Energy&Environment, 2022, 7(3): 372-393. doi: 10.1016/j.gee.2021.05.002
Citation: Zexu Chi, Jingyun Zhao, Yi Zhang, Han Yu, Hongbing Yu. The fabrication of atomically thin-MoS2 based photoanodes for photoelectrochemical energy conversion and environment remediation: A review. Green Energy&Environment, 2022, 7(3): 372-393. doi: 10.1016/j.gee.2021.05.002
shu

The fabrication of atomically thin-MoS2 based photoanodes for photoelectrochemical energy conversion and environment remediation: A review

doi: 10.1016/j.gee.2021.05.002

  • a College of Environment Science and Engineering, Nankai University, Tianjin, 300350, China;

  • b Department of Water Resources Engineering, Lund University, Lund, 22100, Sweden

Funds:

This work was financially supported by the Science and Technology Plans of Tianjin (18PTZWHZ00180), Major National Science and Technology Projects (2017ZX07106001), and Tianjin Development Program for Innovation and Entrepreneurship.

  • Received date 07 March 2021, Accepted date 06 May 2021, RevRecd date 25 April 2021, Publish date 07 May 2021,
    Abstract
  • Photoelectrochemical (PEC) technology has been proved a promising approach to solve the problems of energy shortages and environmental pollution damages. It can convert unlimited solar energy resources into energy forms needed by mankind. The development of highly efficient photoanodes is a key step in realizing the large-scale practical application of PEC systems. However, the development of PEC photoanodes has been severely hindered by the issues of easy recombination of photo-generated charge carriers, low photon-to-electron conversion efficiency, poor photo-corrosion resistance, and low catalytic activity. Therefore, constructing high-performance and stable photoanodes is an urgent research field to promote the progress of PEC technology. The atomically thin molybdenum disulfide (AT-MoS2) with unique physical and chemical properties has been widely applied in the fabrication of PEC photoanodes. The AT-MoS2 based photoanodes have exhibited excellent PEC performance, which providing promising candidates for ideal PEC application. Here, we summarize the fundamental natures of MoS2 and present the research efforts in the preparation of AT-MoS2 based photoanodes. Strategies for the fabrication of high-efficient AT-MoS2 based photoanodes are emphasized to provide guidelines to advance emerging PEC photoanodes. Besides, perspectives for the development of more efficient AT-MoS2 based photoanodes are proposed.

     

    • • AT-MoS2-based photoanode displays promising prospects in the PEC systems. • The fundamental natures and typical preparation methods of AT-MoS2 were summarized. • Strategies for preparing efficient AT-MoS2-based photoanodes were highlighted. • The application of AT-MoS2-based photoanodes in many fields was emphasized. • The perspectives and challenges of AT-MoS2-based photoanode were presented.
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