Volume 8 Issue 1
Feb.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(1): 200-212
Sijia Song, Zipeng Xing, Ke Wang, Huanan Zhao, Peng Chen, Zhenzi Li, Wei Zhou. 3D flower-like mesoporous Bi4O5I2/MoS2 Z-scheme heterojunction with optimized photothermal-photocatalytic performance. Green Energy&Environment, 2023, 8(1): 200-212. doi: 10.1016/j.gee.2021.03.013
Citation: Sijia Song, Zipeng Xing, Ke Wang, Huanan Zhao, Peng Chen, Zhenzi Li, Wei Zhou. 3D flower-like mesoporous Bi4O5I2/MoS2 Z-scheme heterojunction with optimized photothermal-photocatalytic performance. Green Energy&Environment, 2023, 8(1): 200-212. doi: 10.1016/j.gee.2021.03.013
shu

3D flower-like mesoporous Bi4O5I2/MoS2 Z-scheme heterojunction with optimized photothermal-photocatalytic performance

doi: 10.1016/j.gee.2021.03.013

  • a. Department of Environmental Science, School of Chemistry and Materials Science, Key Laboratory of Functional Inorganic Material Chemistry, Ministry of Education of the People's Republic of China, Heilongjiang University, Harbin, 150080, China;

  • b. Shandong Provincial Key Laboratory of Molecular Engineering, School of Chemistry and Chemical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan, Shandong, 250353, China

Funds:

We gratefully acknowledge the support of this research by the National Natural Science Foundation of China (21871078), the Natural Science Foundation of Heilongjiang Province (JQ2019B001 and B2018010), the Heilongjiang Postdoctoral Startup Fund (LBH-Q14135), the Heilongjiang University Science Fund for Distinguished Young Scholars (JCL201802), the Heilongjiang Provincial Institutions of Higher Learning Basic Research Funds Basic Research Projects (KJCX201909), and the Heilongjiang Touyan Innovation Team Program.

  • Received date 06 February 2021, Accepted date 25 March 2021, RevRecd date 18 March 2021, Publish date 27 March 2021,
    Abstract
  • 3D flower-like hierarchical mesoporous Bi4O5I2/MoS2 Z-scheme layered heterojunction photocatalyst was fabricated by oil bath and hydrothermal methods. The heterojunction with narrow band gap of ~1.95 eV extended the photoresponse to near-infrared region, which showed obvious photothermal effect due to the introduction of MoS2 with broad spectrum response. MoS2 nanosheets were anchored onto the surface of flower-like hierarchical mesoporous Bi4O5I2 nanosheets, thereby forming efficient layered heterojunctions, the solar-driven photocatalytic efficiency in degradation of highly toxic dichlorophenol and reduction of hexavalent chromium was improved to 98.5% and 99.2%, which was ~4 and 7 times higher than that of the pristine Bi4O5I2, respectively. In addition, the photocatalytic hydrogen production rate reached 496.78 μmol h-1 g-1, which was ~6 times higher than that of the pristine Bi4O5I2. The excellent photocatalytic performance can be ascribed to the promoted photothermal effect, as well as, the formation of compact Z-scheme layered heterojunctions. The 3D flower-like hierarchical mesoporous structure provided adequate surface active-sites, which was conducive to the mass transfer. Moreover, the high stability of the prepared photocatalyst further promoted its potential practical application. This strategy also provides new insights for fabricating layered Z-scheme heterojunctions photocatalysts with highly photothermal-photocatalytic efficiency.

     

    • • A 3D flower-like mesoporous Bi4O5I2/MoS2 heterojunction is prepared. • It extends the photoresponse from visible light to NIR region. • The mesoporous Bi4O5I2 can provide good hosts to construct layered heterojunctions. • It shows excellent photothermal-photocatalytic performance. • It is due to the formation of Z-scheme layered heterojunctions and 3D flower-like hierarchical mesoporous structure.
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