Volume 7 Issue 4
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Article Navigation >  Green Energy&Environment  > 2022  >  7(4): 662-671
Jingsha Li, Tao Hu, Changhong Wang, Chunxian Guo. Surface-mediated iron on porous cobalt oxide with high energy state for efficient water oxidation electrocatalysis. Green Energy&Environment, 2022, 7(4): 662-671. doi: 10.1016/j.gee.2020.11.009
Citation: Jingsha Li, Tao Hu, Changhong Wang, Chunxian Guo. Surface-mediated iron on porous cobalt oxide with high energy state for efficient water oxidation electrocatalysis. Green Energy&Environment, 2022, 7(4): 662-671. doi: 10.1016/j.gee.2020.11.009
shu

Surface-mediated iron on porous cobalt oxide with high energy state for efficient water oxidation electrocatalysis

doi: 10.1016/j.gee.2020.11.009

  • Institute of Materials Science and Devices, Suzhou University of Science and Technology, Suzhou, 215011, China

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Material.

This work was financially supported by National Natural Science Foundation of China (21972102), Natural Science Foundation of Jiangsu province (BK20200991), Suzhou Science and Technology Planning Project (SS202016), Jiangsu Laboratory for Biochemical Sensing and Biochip, Jiangsu Key Laboratory for Micro and Nano Heat Fluid Flow Technology and Energy Application, Collaborative Innovation Center of Water Treatment Technology &

  • Received date 26 July 2020, Accepted date 18 November 2020, RevRecd date 03 October 2020, Publish date 21 November 2020,
    Abstract
  • Surface engineering of active materials to generate desired energy state is critical to fabricate high-performance heterogeneous catalysts. However, its realization in a controllable level remains challenging. Using oxygen evolution reaction (OER) as a model reaction, we report a surface-mediated Fe deposition strategy to electronically tailor surface energy states of porous Co3O4 (Fe-pCo3O4) for enhanced activity towards OER. The Fe-pCo3O4 exhibits a low overpotential of 280 mV to reach an OER current density of 100 mA cm-2, and a fast-kinetic behavior with a low Tafel slop of 58.2 mV dec-1, outperforming Co3O4-based OER catalysts recently reported and also the noble IrO2. The engineered material retains 100% of its original activity after operating at an overpotential of 350 mV for 100 h. A combination of theoretical calculations and experimental results finds out that the surface doped Fe promotes a high energy state and desired coordination environment in the near surface region, which enables optimized OER intermediates binding and favorably changes the rate-determining step.

     

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