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Xiaojing Fan, Wenwei Sun, Fancheng Meng, Aiming Xing, Jiehua Liu. Advanced chemical strategies for lithium–sulfur batteries: A review. Green Energy&Environment, 2018, 3(1): 2-19. doi: 10.1016/j.gee.2017.08.002
Citation: Xiaojing Fan, Wenwei Sun, Fancheng Meng, Aiming Xing, Jiehua Liu. Advanced chemical strategies for lithium–sulfur batteries: A review. Green Energy&Environment, 2018, 3(1): 2-19. doi: 10.1016/j.gee.2017.08.002
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Advanced chemical strategies for lithium–sulfur batteries: A review

doi: 10.1016/j.gee.2017.08.002

  • Future Energy Laboratory, School of Materials Science and Engineering, Hefei University of Technology, Tunxi Road No.193, Hefei, Anhui, 230009, China

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  • Corresponding author: E-mail address: liujh@hfut.edu.cn (Jiehua Liu)
  • Received date 26 June 2017, Accepted date 19 August 2017, RevRecd date 19 August 2017, Available online 26 August 2017, Publish date 31 January 2018,
    Abstract
  • Lithium–sulfur (LiS) battery has been considered as one of the most promising rechargeable batteries among various energy storage devices owing to the attractive ultrahigh theoretical capacity and low cost. However, the performance of LiS batteries is still far from theoretical prediction because of the inherent insulation of sulfur, shuttling of soluble polysulfides, swelling of cathode volume and the formation of lithium dendrites. Significant efforts have been made to trap polysulfides via physical strategies using carbon based materials, but the interactions between polysulfides and carbon are so weak that the device performance is limited. Chemical strategies provide the relatively complemented routes for improving the batteries' electrochemical properties by introducing strong interactions between functional groups and lithium polysulfides. Therefore, this review mainly discusses the recent advances in chemical absorption for improving the performance of LiS batteries by introducing functional groups (oxygen, nitrogen, and boron, etc.) and chemical additives (metal, polymers, etc.) to the carbon structures, and how these foreign guests immobilize the dissolved polysulfides.

     

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