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Yue Niu, Ziyu Tang, Yan Zhao, Xueyan Zhu, Xiaojing Jia, Jiaming Shao, Andrei Ivanets, Tatyana Kouznetsova, Fawei Lin. Synergistic Electrocatalysis for Enhanced Nitrate Valorization with Dual Strategies of Alternative Anode Reactions and Cathodic Coupling. Green Energy&Environment. doi: 10.1016/j.gee.2026.06.005
Citation: Yue Niu, Ziyu Tang, Yan Zhao, Xueyan Zhu, Xiaojing Jia, Jiaming Shao, Andrei Ivanets, Tatyana Kouznetsova, Fawei Lin. Synergistic Electrocatalysis for Enhanced Nitrate Valorization with Dual Strategies of Alternative Anode Reactions and Cathodic Coupling. Green Energy&Environment. doi: 10.1016/j.gee.2026.06.005
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Synergistic Electrocatalysis for Enhanced Nitrate Valorization with Dual Strategies of Alternative Anode Reactions and Cathodic Coupling

doi: 10.1016/j.gee.2026.06.005

  • 1. School of Environmental Science and Engineering, Tianjin University/Tianjin Key Lab of Biomass/Wastes Utilization, Tianjin 300072, P.R. China;

  • 2. SUPCON Technology Co., Ltd, Hangzhou 310053, P.R. China;

  • 3. State Scientific Institution, “Institute of General and Inorganic Chemistry of National Academy of Sciences of Belarus”, Minsk, 220072, Belarus

Funds:

This work is supported by the National Natural Science Foundation of China (52376205), the Young Elite Scientists Sponsorship Program by CAST (2024-2026QNRC001), and the Young Scientific and Technological Talents (Level Two) in Tianjin (QN20230228).

  • Received date 12 March 2026, Accepted date 07 June 2026, RevRecd date 04 June 2026, Available online 15 June 2026
    Abstract
  • Renewable electricity-driven nitrate reduction reaction (NO3RR) offers a sustainable strategy for simultaneously producing valuable chemicals and reducing environmental pollutants. Traditional systems integrating cathodic NO3RR with anodic oxygen evolution reaction (OER) are severely constrained by the inherent sluggish kinetics of OER, its single reaction pathway, and the low-value products produced, ultimately limiting overall process efficiency and economic viability. Current core solutions focus on two pathways, i.e., replacing OER with thermodynamically more favorable oxidation reactions and directed electrocatalytic coupling between nitrate species and carbon-containing substances at cathodic interfaces. This paper provides a concise review to traditional NO3RR mechanisms and catalyst preparation strategies while categorizing coupled systems into alternative anode coupling and cathodic coupling according to reaction locations. It analyzes mechanistic pathways for directional coupling of nitrates with other carbon-containing substances exemplified by urea formation at the same electrode interface and examines distinct product generation pathways and catalyst design strategies. Additionally, it comprehensively reviews recent advances in coupling cathodic NO3RR with various anodic oxidation reaction (AOR) processes, including reaction variations corresponding to different carbon-chain lengths, novel catalyst preparation strategies with potential mechanisms. Finally, current challenges and future research directions for NO3RR based coupled systems are discussed, aiming to provide scientific guidance for energy-efficient and highly efficient co-production of green ammonia and high-value-added chemicals.

     

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