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Mingxia Wu, Lin Liu, Yu Wang, Siying Zhang, Shutong Liu, Jingxiang Low, Feng Fu, Jun Wan. Recent Advances in High-Entropy Oxides: Composition Modulation, Morphology Control, and Catalytic Applications. Green Energy&Environment. doi: 10.1016/j.gee.2026.05.001
Citation: Mingxia Wu, Lin Liu, Yu Wang, Siying Zhang, Shutong Liu, Jingxiang Low, Feng Fu, Jun Wan. Recent Advances in High-Entropy Oxides: Composition Modulation, Morphology Control, and Catalytic Applications. Green Energy&Environment. doi: 10.1016/j.gee.2026.05.001
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Recent Advances in High-Entropy Oxides: Composition Modulation, Morphology Control, and Catalytic Applications

doi: 10.1016/j.gee.2026.05.001

  • a. College of Chemistry & Chemical Engineering, Shaanxi Key Laboratory of Chemical Reaction Engineering, Clean Utilization of Low Rank Coal of Shaanxi Collaborative Innovation Center, Yan’an University, Yan’an 716000, China;

  • b. School of Physical Science and Technology, Tiangong University, Tianjin, 300387, China

Funds:

Technology Office of Shaanxi Province (2025CY-YBXM-028), and Shaanxi Province Training Program of Innovation and Entrepreneurship for Undergraduates (S202310719069).

This work was supported by the National Natural Science Foundation of China (Nos. 22369023, 22579144), Shaanxi Province Sanqin Talents Introduction Program Project (YJ004), Project of Science &

  • Received date 04 January 2026, Accepted date 07 May 2026, RevRecd date 30 April 2026, Available online 14 May 2026
    Abstract
  • High-entropy oxides (HEOs) have emerged as a promising platform for advanced catalysis owing to their unique structural features, tunable elemental compositions, adjustable functionalities, and four typical synergistic multi-element effects. This review systematically covers HEOs from their fundamental definitions to practical applications, focusing on chemical composition modulation and morphology control through various synthesis approaches that enable precise tailoring of HEO structures. It also analyzes the catalytic performance of HEOs in thermocatalysis, photocatalysis, electrocatalysis, and their synergistic catalytic processes, highlighting their distinct advantages of high catalytic activity, abundant active sites, and exceptional stability. Finally, key challenges and future directions for HEO-based catalysts are outlined, aiming to inspire research efforts in the rational design of HEOs with tailored compositions and morphologies for specific catalytic applications.

     

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