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Ning Wei, Sufeng Zhang, Xue Yao, Scott Renneckar. Entropy-Driven Design of Multifunctional Electrocatalysts: Advances and Perspectives in High-Entropy Materials. Green Energy&Environment. doi: 10.1016/j.gee.2025.10.007
Citation: Ning Wei, Sufeng Zhang, Xue Yao, Scott Renneckar. Entropy-Driven Design of Multifunctional Electrocatalysts: Advances and Perspectives in High-Entropy Materials. Green Energy&Environment. doi: 10.1016/j.gee.2025.10.007
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Entropy-Driven Design of Multifunctional Electrocatalysts: Advances and Perspectives in High-Entropy Materials

doi: 10.1016/j.gee.2025.10.007

  • a. Shaanxi University of Science and Technology, Xi'an, National Demonstration Center for Experimental Light Chemistry Engineering Education, Shaanxi Provincial Key Laboratory of Papermaking Technology and Specialty Paper Development, College of Bioresources Chemical and Materials Engineering, 710021, Shaanxi, China;

  • b. Advanced Renewable Materials Lab, Faculty of Forestry, The University of British Columbia, Vancouver, BC, V6T 1Z4, Canada;

  • c. Bioproducts Institute, Department of Chemical and Biological Engineering, The University of British Columbia, Vancouver, BC V6T 1Z3, Canada

Funds:

This work was supported by the National Natural Science Foundation of China (22378247 and 22078187), China-CEEC University Joint Education Project (2021099), the International Joint Research Center for Biomass Chemistry and Materials, the Shaanxi International Science and Technology Cooperation Base (2018GHJD-19). Ning Wei and Xue Yao are grateful to Innovative Talents International Cooperative Training Project from China Scholarship Council (Grant No. 202310470014 and 202310470013).

  • Received date 06 July 2025, Accepted date 13 October 2025, RevRecd date 05 October 2025, Available online 23 October 2025
    Abstract
  • High-entropy materials (HEMs) have attracted extensive attention in the field of electrocatalysis due to their high performance enabled by their multi-component, tunable structural characteristics and excellent stability. HEMs are usually composed of five or more metal elements, and have core advantages such as high configurational entropy, lattice distortion and multi-element synergistic effect, which provide new possibilities for composition regulation and performance optimization of catalysts. Especially at the nanoscale, HEMs show a larger specific surface area, abundant active sites and higher catalytic reaction efficiency, further expanding their application potential in electrochemical reactions. This paper systematically reviews the classification, structure construction and regulation strategies of HEMs, and focuses on their research progress in critical electrocatalytic reactions including water splitting (HER, OER), hydrogen oxidation (HOR), oxygen reduction (ORR), carbon dioxide reduction (CO2RR), nitrate reduction (NO3–RR) and electrooxidation of organics (EOO). In addition, the preparation methods of HEMs, the structure-performance relationship and the entropy regulation mechanism in the catalytic process are analyzed. Finally, this paper proposes the key challenges currently faced by HEMs in electrocatalytic applications and looks forward to their future development direction, providing a theoretical basis and design ideas for building a new generation of efficient and sustainable electrocatalysts.

     

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