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Yunxin Shi, Ziyang Guo, Changhong Wang, Mingze Gao, Xiaoting Lin, Hui Duan, Yonggang Wang, Xueliang Sun. Design of Multifunctional Interfaces on Ceramic Solid Electrolytes for High-Performance Lithium-Air Batteries. Green Energy&Environment. doi: 10.1016/j.gee.2024.02.010
Citation: Yunxin Shi, Ziyang Guo, Changhong Wang, Mingze Gao, Xiaoting Lin, Hui Duan, Yonggang Wang, Xueliang Sun. Design of Multifunctional Interfaces on Ceramic Solid Electrolytes for High-Performance Lithium-Air Batteries. Green Energy&Environment. doi: 10.1016/j.gee.2024.02.010
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Design of Multifunctional Interfaces on Ceramic Solid Electrolytes for High-Performance Lithium-Air Batteries

doi: 10.1016/j.gee.2024.02.010

  • a. College of Energy Material and Chemistry, College of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, P.R. China;

  • b. Department of Mechanical and Materials Engineering, Western University, London, ON, N6A 5B9, Canada;

  • c. Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Institute of New Energy, iChEM(Collaborative Innovation Center of Chemistry for Energy Materials), Fudan University, Shanghai 200433, China;

  • d. Eastern Institute for Advanced Study, Eastern Institute of Technology, Ningbo, Zhejiang, 315100, China

  • Received date 09 January 2024, Accepted date 28 February 2024, RevRecd date 20 February 2024, Available online 02 March 2024
    Abstract
  • High-energy-density lithium (Li)-air cells have been considered a promising energy-storage system, but the liquid electrolyte-related safety and side-reaction problems seriously hinder their development. To address these above issues, solid-state Li-air batteries have been widely developed. However, many commonly-used solid electrolytes generally face huge interface impedance in Li-air cells and also show poor stability towards ambient air/Li electrodes. Herein, we fabricate a differentiating surface-regulated ceramic-based composite electrolyte (DSCCE) by constructing disparately LiI-containing polymethyl methacrylate (PMMA) coating and Poly(vinylidene fluoride-co-hexafluoropropylene) (PVDF-HFP) layer on both sides of Li1.5Al0.5Ge1.5(PO4)3 (LAGP). The cathode-friendly LiI/PMMA layer displays excellent stability towards O2- and also greatly reduces the decomposition voltage of discharge products in Li-air system. Additionally, the anode-friendly PVDF-HFP coating shows low-resistance properties towards anodes.Moreover, Li dendrite/passivation derived from liquid electrolyte-induced side reactions and air/I-attacking can be obviously suppressed by the uniform and compact composite framework. As a result, the DSCCE-based Li-air batteries possess high capacity/low voltage polarization (11836 mA h g-1/1.45 V under 500 mA g-1), good rate performance (capacity ratio under 1000 mA g-1/250 mA g-1 is 68.2 %) and long-term stable cell operation (300 cycles at 750 mA g-1 with 750 mAh g-1) in ambient air.

     

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