Volume 9 Issue 6
Jun.  2024
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Article Navigation >  Green Energy&Environment  > 2024  >  9(6): 937-948
Yibo Liu, Xing Hu, Chenxi Liu, Shan Zhu, Kezhu Jiang, Feng Liu, Shijian Zheng. Construction of Pd-doped RuO2 nanosheets for efficient and stable acidic water oxidation. Green Energy&Environment, 2024, 9(6): 937-948. doi: 10.1016/j.gee.2023.12.003
Citation: Yibo Liu, Xing Hu, Chenxi Liu, Shan Zhu, Kezhu Jiang, Feng Liu, Shijian Zheng. Construction of Pd-doped RuO2 nanosheets for efficient and stable acidic water oxidation. Green Energy&Environment, 2024, 9(6): 937-948. doi: 10.1016/j.gee.2023.12.003
shu

Construction of Pd-doped RuO2 nanosheets for efficient and stable acidic water oxidation

doi: 10.1016/j.gee.2023.12.003

  • a. Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, College of Materials Science and Engineering, Hebei University of Technology, Tianjin, 300401, China;

  • b. Yunnan Precious Metals Lab Co., LTD, Kunming, 650100, China

Funds:

This work was supported by the National Natural Science Foundation of China (No. 22209035), the Major Science and Technology Projects of Yunnan Province (No. 202302AH360001), and the Natural Science Foundation of Hebei Province (No. E2020202091). We thank Shenzhen HUASUAN Technology Co., Ltd., for performing the DFT calculations and data analysis.

  • Received date 15 August 2023, Accepted date 03 December 2023, RevRecd date 14 November 2023, Publish date 13 December 2023,
    Abstract
  • RuO2 has been considered a potential alternative to commercial IrO2 for the oxygen evolution reaction (OER) due to its superior intrinsic activity. However, its inherent structure dissolution in acidic environments restricts its commercial applications. In this study, we report a novel Pd-doped ruthenium oxide (Pd-RuO2) nanosheet catalyst that exhibits improved activity and stability through a synergistic effect of Pd modulation of Ru electronic structure and the two-dimensional structure. The catalyst exhibits excellent performance, achieving an overpotential of only 204 mV at a current density of 10 mA cm-2. Impressively, after undergoing 8000 cycles of cyclic voltammetry testing, the overpotential merely decreased by 5 mV. The PEM electrolyzer with Pd0.08Ru0.92O2 as an anode catalyst survived an almost 130 h operation at 200 mA cm-2. To elucidate the underlying mechanisms responsible for the enhanced stability, we conducted an X-ray photoelectron spectroscopy (XPS) analysis, which reveals that the electron transfer from Pd to Ru effectively circumvents the over-oxidation of Ru, thus playing a crucial role in enhancing the catalyst's stability. Furthermore, density functional theory (DFT) calculations provide compelling evidence that the introduction of Pd into RuO2 effectively modulates electron correlations and facilitates the electron transfer from Pd to Ru, thereby preventing the over-oxidation of Ru. Additionally, the application of the two-dimensional structure effectively inhibited the aggregation and growth of nanoparticles, further bolstering the structural integrity of the catalyst.

     

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