Volume 8 Issue 6
Dec.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(6): 1501-1508
Baiyi Chen, Huimeng Wang, Jiadai Xu, Liting Pan, Yuan Jing, Xu Hou. Temperature-regulation liquid gating membrane with controllable gas/liquid separation. Green Energy&Environment, 2023, 8(6): 1501-1508. doi: 10.1016/j.gee.2023.04.002
Citation: Baiyi Chen, Huimeng Wang, Jiadai Xu, Liting Pan, Yuan Jing, Xu Hou. Temperature-regulation liquid gating membrane with controllable gas/liquid separation. Green Energy&Environment, 2023, 8(6): 1501-1508. doi: 10.1016/j.gee.2023.04.002
shu

Temperature-regulation liquid gating membrane with controllable gas/liquid separation

doi: 10.1016/j.gee.2023.04.002

  • a. State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China;

  • b. Department of Physics, Research Institute for Biomimetics and Soft Matter, Fujian Provincial Key Laboratory for Soft Functional Materials Research, Jiujiang Research Institute, College of Physical Science and Technology, Xiamen University, Xiamen, 361005, China;

  • c. Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (IKKEM), Xiamen, 361102, China;

  • d. State Key Laboratory of Bio-Fibers and Eco-Textiles, Qingdao University, Qingdao, 266071, China

Funds:

This work was supported by the National Natural Science Foundation of China (52025132, 21621091, 22021001, 22121001, 22275207 and T2241022), the National Science Foundation of Fujian Province of China (2022J02059), the State Key Laboratory of Bio-Fibers and Eco-Textiles (Qingdao University) (KFKT202221), the 111 Project (B17027, B16029), the Science and Technology Projects of Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (RD2022070601), the Tencent Foundation (The XPLORER PRIZE).

  • Received date 11 January 2023, Accepted date 08 April 2023, RevRecd date 20 March 2023, Publish date 11 April 2023,
    Abstract
  • Membrane separation technology with the ability to regulate gas/liquid transport and separation is critical for environmental fields, such as sewerage treatment, multiphase separation, and desalination. Although numerous membranes can dynamically control liquid-phase fluids transport via external stimuli, the transport and separation of gas-phase fluids remains a challenge. Here, we show a temperature-regulation liquid gating membrane that allows in-situ dynamically controllable gas/liquid transfer and multiphase separation by integrating a thermo-wettability responsive porous membrane with functional gating liquid. Experiments and theoretical analysis have demonstrated the temperature-regulation mechanism of this liquid gating system, which is based on thermo-responsive changes of porous membrane surface polarity, leading to changes in affinity between the porous membrane and the gating liquid. In addition, the sandwich configuration with dense Au-coated surfaces and heterogeneous internal components by a bistable interface design enables the liquid gating system to enhance response sensitivity and maintain working stability. This temperature-regulation gas/liquid transfer strategy expands the application range of liquid gating membranes, which are promising in environmental governance, water treatment and multiphase separation.

     

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