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Article Navigation >  Green Energy&Environment  > 2023  > Accepted Manuscript
Yunchen Ge, Yan Meng, Lin Liu, Jianming Li, Xuechun Huang, Dan Xiao. Mechanochemical strategy assisted morphology recombination of COFs for promoted kinetics and LiPS transformation in Li-S batteries. Green Energy&Environment. doi: 10.1016/j.gee.2023.03.005
Citation: Yunchen Ge, Yan Meng, Lin Liu, Jianming Li, Xuechun Huang, Dan Xiao. Mechanochemical strategy assisted morphology recombination of COFs for promoted kinetics and LiPS transformation in Li-S batteries. Green Energy&Environment. doi: 10.1016/j.gee.2023.03.005
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Mechanochemical strategy assisted morphology recombination of COFs for promoted kinetics and LiPS transformation in Li-S batteries

doi: 10.1016/j.gee.2023.03.005

  • a Institute of New Energy and Low-Carbon Technology(INELT), Sichuan University, Chengdu 610000, Sichuan, PR China;

  • b School of Chemical Engineering and College of Chemistry, Sichuan University, Chengdu 610065, Sichuan, PR China

Funds:

This work is supported by the National Natural Science Foundation of China (Nos. 81927809).

  • Received date 24 February 2023, Accepted date 27 March 2023, RevRecd date 22 March 2023, Available online 18 April 2023
    Abstract
  • A covalent organic frameworks (COFs) material with regular pores and stable structure can be used as the host of lithium-sulfur batteries to improve battery kinetics and polysulfides conversion. Herein, we designed and synthesized two kinds of rod-liked bulk COFs by adjusting different pore sizes (COF-BTD and COF-TFB), unfortunately, the active sites masking and sluggish kinetics have not met our expectations. Generally, the available layered COFs prepared from mechanochemical can expose abundant active sites and favorable kinetics than bulk COFs. Thus, simple mechanical ball milling is applied to activate the above COFs (M-COFs group). It is worth noting that layered R-COF-BTD is directly synthesized from rod-liked precursors by simple morphological reconstruction. A series of characterization methods are used to systematically explore the advantages of the group of M-COFs@S electrodes in the cycling process, including the effects of specific morphology on the kinetics and transformation of polysulfides. Our research provides a feasible plan for the development and selection of the host material of lithium-sulfur batteries.

     

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