Volume 9 Issue 7
Jul.  2024
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Article Navigation >  Green Energy&Environment  > 2024  >  9(7): 1159-1170
Liquan Jing, Meng Xie, Yuanguo Xu, Chun Tong, Xia Du, Heng Zhao, Na Zhong, Huaming Li, Jinguang Hu. Advanced oxidation via the synergy of C-defective/ C–O band modified ultrathin porous g-C3N4 and PMS for efficient photothermal degradation of bisphenol pollutants and lignin derivatives. Green Energy&Environment, 2024, 9(7): 1159-1170. doi: 10.1016/j.gee.2023.01.006
Citation: Liquan Jing, Meng Xie, Yuanguo Xu, Chun Tong, Xia Du, Heng Zhao, Na Zhong, Huaming Li, Jinguang Hu. Advanced oxidation via the synergy of C-defective/ C–O band modified ultrathin porous g-C3N4 and PMS for efficient photothermal degradation of bisphenol pollutants and lignin derivatives. Green Energy&Environment, 2024, 9(7): 1159-1170. doi: 10.1016/j.gee.2023.01.006
shu

Advanced oxidation via the synergy of C-defective/ C–O band modified ultrathin porous g-C3N4 and PMS for efficient photothermal degradation of bisphenol pollutants and lignin derivatives

doi: 10.1016/j.gee.2023.01.006

  • a. School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013, China;

  • b. Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Drive, NW, Calgary, Alberta, T2N1N4, Canada;

  • c. School of Pharmacy, Jiangsu University, Zhenjiang, 212013, China;

  • d. School of Material Science & Chemical Engineering, Harbin University of Science and Technology, Harbin, 150080, China;

  • e. Institute for Energy Research, Jiangsu University, Zhenjiang, 212013, China

Funds:

The authors thank the National Natural Science Foundation of China (No. 22076068, 8111310014) (China) and the University of Calgary’s Canada First Research Excellence Fund (CFREF) program (Canada) for financial support.

  • Received date 30 November 2022, Accepted date 27 January 2023, RevRecd date 12 January 2023, Publish date 31 July 2024,
    Abstract
  • This work uses thermal polymerization of urea nitrate, oxyacetic acid and urea as the raw material to prepare ultra-thin porous carbon nitride with carbon defects and C–O band (OA-UN-CN). Density functional theory (DFT) calculations showed OA-UN-CN had narrower band gap, faster electron transport and a new internal construction electric field. Additionally, the prepared OA-UN-CN significantly enhanced photocatalytic activation of peroxymonosulfate (PMS) due to enhanced light absorption performance and faster electron overflow. As the result, the OA-UN-CN/PMS could entirely degrade bisphenol A (BPA) within 30 min, where the photodegradation rate was 81.8 and 7.9 times higher than that of g-C3N4 and OA-UN-CN, respectively. Beyond, the OA-UN-CN/PMS could likewise degrade other bisphenol pollutants and sodium lignosulfonate efficiently. We suggested possible photocatalytic degradation pathways accordingly and explored the toxicity of its degradation products. This work provides a new idea on the development of advanced photocatalytic oxidation processes for the treatment of bisphenol pollutants and lignin derivatives, via a metal-free photothermal-catalyst.

     

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