Volume 9 Issue 7
Jul.  2024
Turn off MathJax
Article Contents
Article Navigation >  Green Energy&Environment  > 2024  >  9(7): 1159-1170
Liquan Jing, Meng Xie, Yuanguo Xu, Chun Tong, Xia Du, Heng Zhao, Na Zhong, Huaming Li, Jinguang Hu. Advanced oxidation via the synergy of C-defective/ C–O band modified ultrathin porous g-C3N4 and PMS for efficient photothermal degradation of bisphenol pollutants and lignin derivatives. Green Energy&Environment, 2024, 9(7): 1159-1170. doi: 10.1016/j.gee.2023.01.006
Citation: Liquan Jing, Meng Xie, Yuanguo Xu, Chun Tong, Xia Du, Heng Zhao, Na Zhong, Huaming Li, Jinguang Hu. Advanced oxidation via the synergy of C-defective/ C–O band modified ultrathin porous g-C3N4 and PMS for efficient photothermal degradation of bisphenol pollutants and lignin derivatives. Green Energy&Environment, 2024, 9(7): 1159-1170. doi: 10.1016/j.gee.2023.01.006
shu

Advanced oxidation via the synergy of C-defective/ C–O band modified ultrathin porous g-C3N4 and PMS for efficient photothermal degradation of bisphenol pollutants and lignin derivatives

doi: 10.1016/j.gee.2023.01.006

  • a. School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang, 212013, China;

  • b. Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Drive, NW, Calgary, Alberta, T2N1N4, Canada;

  • c. School of Pharmacy, Jiangsu University, Zhenjiang, 212013, China;

  • d. School of Material Science & Chemical Engineering, Harbin University of Science and Technology, Harbin, 150080, China;

  • e. Institute for Energy Research, Jiangsu University, Zhenjiang, 212013, China

Funds:

The authors thank the National Natural Science Foundation of China (No. 22076068, 8111310014) (China) and the University of Calgary’s Canada First Research Excellence Fund (CFREF) program (Canada) for financial support.

  • Received date 30 November 2022, Accepted date 27 January 2023, RevRecd date 12 January 2023, Publish date 31 July 2024,
    Abstract
  • This work uses thermal polymerization of urea nitrate, oxyacetic acid and urea as the raw material to prepare ultra-thin porous carbon nitride with carbon defects and C–O band (OA-UN-CN). Density functional theory (DFT) calculations showed OA-UN-CN had narrower band gap, faster electron transport and a new internal construction electric field. Additionally, the prepared OA-UN-CN significantly enhanced photocatalytic activation of peroxymonosulfate (PMS) due to enhanced light absorption performance and faster electron overflow. As the result, the OA-UN-CN/PMS could entirely degrade bisphenol A (BPA) within 30 min, where the photodegradation rate was 81.8 and 7.9 times higher than that of g-C3N4 and OA-UN-CN, respectively. Beyond, the OA-UN-CN/PMS could likewise degrade other bisphenol pollutants and sodium lignosulfonate efficiently. We suggested possible photocatalytic degradation pathways accordingly and explored the toxicity of its degradation products. This work provides a new idea on the development of advanced photocatalytic oxidation processes for the treatment of bisphenol pollutants and lignin derivatives, via a metal-free photothermal-catalyst.

     

    • FullText(HTML)
  • loading
    • References(74)
  • [1]
    R. Banaderakhshan, P. Kemp, L. Breul, P. Steinbichl, C. Hartmann, M. Fürhacker, Chemosphere 286(2022)131842.
    [2]
    R. Zhong, H. He, M. Jin, Z. Lu, Y. Deng, C. Liu, N. Shen, J. Li, H. Wang, P. Ying, B. Li, Q. Zeng, Q. Lu, L. Cheng, Y. Zhu, X. Miao, J. Tian, Sci. Total Environ. 807(2022)150753.
    [3]
    X.-Y. Pei, H.-Y. Ren, G.-S. Liu, G.-L. Cao, G.-J. Xie, D.-F. Xing, N.-Q. Ren, B.-F. Liu, J. Hazard Mater. 424(2022)127254.
    [4]
    J. Jia, D. Liu, Q. Wang, H. Li, J. Ni, F. Cui, J. Tian, J. Hazard Mater. 424(2022)127434.
    [5]
    L. Xu, Y. Hu, Q. Zhu, C. Liao, G. Jiang, J. Hazard Mater. 424(2022)127489.
    [6]
    X. Liu, Q. Xue, H. Zhang, J. Fu, A. Zhang, Sci. Total Environ. 793(2021)148558.
    [7]
    P. Dualde, O. Pardo, F. Corpas-Burgos, J. Kuligowski, M. Gormaz, M. Vento, A. Pastor, V. Yusà, Sci. Total Environ. 668(2019)797-805.
    [8]
    C. Guo, F. Ren, J. Jin, H. Zhang, L. Wang, H. Zhang, J. Chen, Environ. Int. 156(2021)106759.
    [9]
    J. Chen, W. Liu, Z. Song, H. Wang, Y. Xie, BioEnergy Research 11(2018)166-173.
    [10]
    R. Chen, Y. Huang, C. Rao, H. Su, Y. Pang, H. Lou, D. Yang, X. Qiu, Appl. Surf. Sci. 600(2022)154110.
    [11]
    L. Jing, M. Xie, Y. Xu, C. Tong, H. Zhao, N. Zhong, H. Li, I.D. Gates, J. Hu, Appl. Catal. B Environ. 318(2022)121814.
    [12]
    W. Zhang, L. Yan, Q. Wang, X. Li, Y. Guo, W. Song, Y. Li, J. Environ. Chem. Eng. 9(2021)106870.
    [13]
    Y. Zhao, X. Zhan, H. Wang, J. Yu, Y. Sun, L. Chen, M. He, J. Liu, H. Shi, Chem. Eng. J. 433(2022)133806.
    [14]
    X. Dou, Y. Chen, H. Shi, Chem. Eng. J. 431(2022)134054.
    [15]
    Q. Han, M. Wang, F. Sun, B. Yu, Z. Dong, P. Li, J. Luo, M. Li, X. Jin, Z. Dai, Environ. Res. 216(2023)114601.
    [16]
    M. Zhang, Y. Li, B. Yang, Y. Su, J. Xu, J. Deng, T. Zhou, Separ. Purif. Technol. 306(2023)122566.
    [17]
    J. Wang, J. Yao, L. Zhu, C. Gao, J. Liu, S. She, X. Wu, Chemosphere 289(2022)133211.
    [18]
    H. Liu, J. Liang, X. Du, R. Wang, T. Tang, X. Tao, H. Yin, Z. Dang, G. Lu, Sci. Total Environ. 809(2022)152185.
    [19]
    X. Zheng, X. Zhang, Y. Cai, S. Zhao, S. Wang, Chemosphere 289(2022)133158.
    [20]
    Y. He, J. Qian, P. Wang, J. Wu, B. Lu, S. Tang, P. Gao, Chem. Eng. J. 431(2022)133933.
    [21]
    S. Li, Z. Jin, X. Jiang, J. Yu, Y. Wang, S. Jin, H. Zhang, S. Song, T. Zeng, Chem. Eng. J. 431(2022)133900.
    [22]
    D. Wang, J. Chen, X. Gao, Y. Ao, P. Wang, Chem. Eng. J. 431(2022)134105.
    [23]
    H. Shi, Y. He, Y. Li, T. He, P. Luo, Separ. Purif. Technol. 280(2022)119864.
    [24]
    Z. Jin, S. Li, S. Jin, D. Wang, F. Dong, S. Song, M. Liu, T. Zeng, Catal. Commun. 171(2022)106512.
    [25]
    M. Wang, J. Kang, S. Li, J. Zhang, Y. Tang, S. Liu, J. Liu, P. Tang, Chem. Eng. J. 436(2022)135278.
    [26]
    K. Xu, K. Cui, M. Cui, X. Liu, X. Chen, X. Tang, X. Wang, Separ. Purif. Technol. 294(2022)121246.
    [27]
    K. Li, Y. Jiang, W. Rao, Y. Li, X. Liu, J. Zhang, X. Xu, K. Lin, Chem. Eng. J. 431(2022)134075.
    [28]
    X.-B. Ding, F. Li, Q.-C. Cao, H. Wu, Y.-H. Qin, L. Yang, T. Wang, X. Zheng, C.-W. Wang, Chem. Eng. J. 429(2022)132469.
    [29]
    X. Mei, S. Chen, G. Wang, W. Chen, W. Lu, B. Zhang, Y. Fang, C. Qi, J. Solid State Chem. 310(2022)123053.
    [30]
    Y. Meng, Z. Li, J. Tan, J. Li, J. Wu, T. Zhang, X. Wang, Chem. Eng. J. 429(2022)130860.
    [31]
    Y. Zhu, Z. Chen, Y. Gao, C. Hu, J. Hazard Mater. 394(2020)122578.
    [32]
    J. Cao, W. Nie, L. Huang, Y. Ding, K. Lv, H. Tang, Appl. Catal. B Environ. 241(2019)18-27.
    [33]
    L. Jing, D. Wang, Y. Xu, M. Xie, J. Yan, M. He, Z. Song, H. Xu, H. Li, J. Colloid Interface Sci. 566(2020)171-182.
    [34]
    H. Che, P. Wang, J. Chen, X. Gao, B. Liu, Y. Ao, Appl. Catal. B Environ. 316(2022)121611.
    [35]
    B. He, M. Feng, X. Chen, J. Sun, Green Energy Environ. 6(2021)823-845.
    [36]
    X. Zhang, W. Yang, M. Gao, H. Liu, K. Li, Y. Yu, Green Energy Environ. 7(2022)66-74.
    [37]
    W. Zhang, J. Wang, Z. Liu, Y. Pi, R. Tan, Green Energy Environ. 7(2022)712-722.
    [38]
    D. Yuan, Z. Li, X. Chen, J. Ding, H. Wan, G. Guan, Green Energy Environ. 7(2022)1119-1127.
    [39]
    S. Dong, M. Chen, J. Zhang, J. Chen, Y. Xu, Green Energy Environ. 6(2021)715-724.
    [40]
    J. Tan, Z. Li, J. Li, Y. Meng, X. Yao, Y. Wang, Y. Lu, T. Zhang, J. Hazard. Mater. 423(2022)127048.
    [41]
    W. Jiang, Q. Ruan, J. Xie, X. Chen, Y. Zhu, J. Tang, Appl. Catal. B Environ. 236(2018)428-435.
    [42]
    F. Li, M. Han, Y. Jin, L. Zhang, T. Li, Y. Gao, C. Hu, Appl. Catal. B Environ. 256(2019)117705.
    [43]
    Y. Yu, S. Wu, J. Gu, R. Liu, Z. Wang, H. Chen, F. Jiang, J. Hazard Mater. 384(2020)121247.
    [44]
    Y. Wang, F. Silveri, M.K. Bayazit, Q. Ruan, Y. Li, J. Xie, C.R.A. Catlow, J. Tang, Adv. Energy Mater. 8(2018)1801084.
    [45]
    M. Wu, X. He, B. Jing, T. Wang, C. Wang, Y. Qin, Z. Ao, S. Wang, T. An, J. Hazard Mater. 384(2020)121323.
    [46]
    S. Su, Z. Xing, S. Zhang, M. Du, Y. Wang, Z. Li, P. Chen, Q. Zhu, W. Zhou, Appl. Surf. Sci. 537(2021)147890.
    [47]
    F. Zhang, L. Yang, H. Yan, B. Tian, X. Zhu, J. Mater. Chem. B 10(2022)9923-9930.
    [48]
    B. Yan, C. Du, Z. Lin, G. Yang, Phys. Chem. Chem. Phys. 22(2020)4453-4463. L. Jing et al./Green Energy&Environment 9(2024)1159-11701169
    [49]
    Z. Li, H. Bai, J. Wei, J. Wang, L. Kong, X. Wang, X. Xia, J. Duan, J. Colloid Interface Sci. 610(2022)893-904.
    [50]
    S. Tang, S. Yang, Y. Chen, Y. Yang, Z. Li, L. Zi, Y. Liu, Y. Wang, Z. Li, Z. Fu, Y. Li, Carbon 201(2023)815-828.
    [51]
    Y. Jiang, C. Cao, Y. Tan, Q. Chen, L. Zeng, W. Yang, Z. Sun, L. Huang, J. Mater. Sci. Technol. 141(2023)32-41.
    [52]
    Z. Ma, X. Zong, Q. Hong, L. Niu, T. Yang, W. Jiang, D. Qu, L. An, X. Wang, Z. Kang, Z. Sun, Appl. Catal. B Environ. 319(2022)121922.
    [53]
    M. Ai, L. Pan, Y. Chen, C. Shi, Z.-F. Huang, X, X. Zhang, J.-J. Zou, J. Catal. 418(2023)22-30.
    [54]
    Y. Zheng, Y. Luo, Q. Ruan, S. Wang, J. Yu, X. Guo, W. Zhang, H. Xie, Z. Zhang, Y. Huang, Appl. Catal. B Environ. 311(2022)121372.
    [55]
    W. Wang, S.-P. Gao, Int. J. Hydrogen Energy 47(2022)8761-8775.
    [56]
    N. Minhas, G. Mustafa, K. Kaur, N. Kaur, G. Singh, A. Kaura, J.K. Goswamy, J. Phys. Chem. Solid. 170(2022)110905.
    [57]
    Y. Zhou, J. He, J. Lu, Y. Liu, Y. Zhou, Chin. Chem. Lett. 31(2020)2623-2626.
    [58]
    N. Klüver, C. Vogs, R. Altenburger, B.I. Escher, S. Scholz, Chemosphere 164(2016)164-173.
    [59]
    B. Peric, J. Sierra, E. Martí, R. Cruañas, M.A. Garau, Ecotoxicol. Environ. Saf. 115(2015)257-262.
    [60]
    K. Grabicova, R. Grabic, G. Fedorova, J. Fick, D. Cerveny, J. Kolarova, J. Turek, V. Zlabek, T. Randak, Water Res. 124(2017)654-662.
    [61]
    R. Guo, Y. Du, F. Zheng, J. Wang, Z. Wang, R. Ji, J. Chen, Environ. Pollut. 227(2017)460-467.
    [62]
    M. Iqbal, I.A. Bhatti, J. Hazard Mater. 299(2015)351-360.
    [63]
    C. Tong, L. Jing, M. Xie, M. He, Y. Liu, J. Yuan, Y. Song, Y. Xu, J. Hazard Mater. 432(2022)128663.
    [64]
    J. Zhang, X. Zhao, Y. Wang, Y. Gong, D. Cao, M. Qiao, Appl. Catal. B Environ. 237(2018)976-985.
    [65]
    H. Ming, D. Wei, Y. Yang, B. Chen, C. Yang, J. Zhang, Y. Hou, Chem. Eng. J. 424(2021)130296.
    [66]
    H. Wang, W. Guo, Q. Si, B. Liu, Q. Zhao, H. Luo, N. Ren, Chem. Eng. J. 418(2021)129504.
    [67]
    M. Cui, K. Cui, X. Liu, X. Chen, Y. Chen, Z. Guo, J. Hazard Mater. 424(2022)127292.
    [68]
    Q. Jiang, H. Gan, Y. Huang, D. Lu, Y. Yang, W. Zhang, J. Environ. Chem. Eng. 9(2021)106592.
    [69]
    H. Ming, P. Zhang, Y. Yang, Y. Zou, C. Yang, Y. Hou, K. Ding, J. Zhang, X. Wang, Appl. Catal. B Environ. 311(2022)121341.
    [70]
    C. Dong, Z. Zheng, Z. Wang, J. He, Z. Ye, X. Gong, I.M.C. Lo, J. Hazard Mater. 416(2021)125891.
    [71]
    J. Li, W. Huang, L. Yang, G. Gou, C. Zhou, L. Li, N. Li, C. Liu, B. Lai, Chem. Eng. J. 432(2022)133588.
    [72]
    Y. Deng, L. Li, H. Zeng, R. Tang, Z. Zhou, Y. Sun, C. Feng, D. Gong, J. Wang, Y. Huang, Chem. Eng. J. 457(2023)141261.
    [73]
    X. Zhang, B. Xu, X. Li, X. Fan, J. Zhang, Y. Yu, Y. Sun, Chem. Eng. J. 457(2023)141219.
    [74]
    A. Sudhaik, P. Raizada, S. Thakur, A.K. Saini, P. Singh, A. HosseiniBandegharaei, Mater. Lett. 277(2020)128277.
    • Relative Articles
    • Supplements(0)
    • Cited By
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Get Citation
    PDF
    XML

    Article Metrics

    Article views (355) PDF downloads(35) Cited by()
    Proportional views

    Publish With GEE

    Contact

    • Email：gee@ipe.ac.cn
    • Tel：010-82627075
    • Address：North 2nd street, Zhongguancun, Haidian District, Beijing, China

    Links

    京ICP备10002620号-1京公网安备 11010802039050号

    Supported by: Beijing Renhe Information Technology Co. Ltd    

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return