Volume 8 Issue 5
Oct.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(5): 1488-1500
Yao Qiu, Chunjie Zhang, Rui Zhang, Zhiyuan Liu, Huazeng Yang, Shuai Qi, Yongzhao Hou, Guangwu Wen, Jilei Liu, Dong Wang. Integration of pore structure modulation and B, N co-doping for enhanced capacitance deionization of biomass-derived carbon. Green Energy&Environment, 2023, 8(5): 1488-1500. doi: 10.1016/j.gee.2023.01.005
Citation: Yao Qiu, Chunjie Zhang, Rui Zhang, Zhiyuan Liu, Huazeng Yang, Shuai Qi, Yongzhao Hou, Guangwu Wen, Jilei Liu, Dong Wang. Integration of pore structure modulation and B, N co-doping for enhanced capacitance deionization of biomass-derived carbon. Green Energy&Environment, 2023, 8(5): 1488-1500. doi: 10.1016/j.gee.2023.01.005
shu

Integration of pore structure modulation and B, N co-doping for enhanced capacitance deionization of biomass-derived carbon

doi: 10.1016/j.gee.2023.01.005

  • a. School of Materials Science and Engineering, Shandong University of Technology, 266 Xincun West Road, Zibo, 255000, China;

  • b. School of Materials Science and Engineering, Harbin Institute of Technology, 92 Xidazhi Street, Harbin, 150001, China;

  • c. College of Chemistry and Environmental Engineering, Shenzhen University, 1066 Xueyuan Ave, Shenzhen, 518060, China;

  • d. College of Materials Science and Engineering, Hunan University, 2 South Lushan Road, Changsha, 410082, China

Funds:

We gratefully acknowledge financial supports from the National Natural Science Foundation of China (No. 52202371, 51905125, 52102364), the Natural Science Foundation of Shandong Province (No. ZR2020QE066), Opening Project of State Key Laboratory of Advanced Technology for Float Glass (No. 2020KF08), SDUT&Zibo City Integration Development Project (No. 2021SNPT0045), the fellowship of China Postdoctoral Science Foundation (No. 2020M672081).

  • Received date 05 November 2022, Accepted date 18 January 2023, RevRecd date 25 December 2022, Publish date 20 January 2023,
    Abstract
  • Biomass-derived carbon has demonstrated great potentials as advanced electrode for capacitive deionization (CDI), owing to good electroconductivity, easy availability, intrinsic pores/channels. However, conventional simple pyrolysis of biomass always generates inadequate porosity with limited surface area. Moreover, biomass-derived carbon also suffers from poor wettability and single physical adsorption of ions, resulting in limited desalination performance. Herein, pore structure optimization and element co-doping are integrated on banana peels (BP)-derived carbon to construct hierarchically porous and B, N co-doped carbon with large ions-accessible surface area. A unique expansion-activation (EA) strategy is proposed to modulate the porosity and specific surface area of carbon. Furthermore, B, N co-doping could increase the ions-accessible sites with improved hydrophilicity, and promote ions adsorption. Benefitting from the synergistic effect of hierarchical porosity and B, N co-doping, the resultant electrode manifest enhanced CDI performance for NaCl with large desalination capacity (29.5 mg g−1), high salt adsorption rate (6.2 mg g−1 min−1), and versatile adsorption ability for other salts. Density functional theory reveals the enhanced deionization mechanism by pore and B, N co-doping. This work proposes a facile EA strategy for pore structure modulation of biomass-derived carbon, and demonstrates great potentials of integrating pore and heteroatoms-doping on constructing high-performance CDI electrode.

     

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