Volume 9 Issue 3
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Article Navigation >  Green Energy&Environment  > 2024  >  9(3): 516-528
Miaomiao Hu, Kun Zhou, Tingyi Zhao, Zheng Li, Xianhai Zeng, Di Yu, Xuehua Yu, Mingqin Zhao, Zhihui Shao, Qixiang Xu, Bing Cui. Facile preparation and efficient MnxCoy porous nanosheets for the sustainable catalytic process of soot. Green Energy&Environment, 2024, 9(3): 516-528. doi: 10.1016/j.gee.2022.08.006
Citation: Miaomiao Hu, Kun Zhou, Tingyi Zhao, Zheng Li, Xianhai Zeng, Di Yu, Xuehua Yu, Mingqin Zhao, Zhihui Shao, Qixiang Xu, Bing Cui. Facile preparation and efficient MnxCoy porous nanosheets for the sustainable catalytic process of soot. Green Energy&Environment, 2024, 9(3): 516-528. doi: 10.1016/j.gee.2022.08.006
shu

Facile preparation and efficient MnxCoy porous nanosheets for the sustainable catalytic process of soot

doi: 10.1016/j.gee.2022.08.006

  • a. Flavors and Fragrance Engineering & Technology Research Center of Henan Province, College of Tobacco Science, Henan Agricultural University, Zhengzhou, 450002, China;

  • b. School of Ecology and Environment, Zhengzhou University, Zhengzhou, 450001, China;

  • c. College of Energy, Xiamen University, Xiamen, 361102, China;

  • d. College of Chemistry and Chemical Engineering, Shenyang Normal University, Shenyang, 110034, China

Funds:

This work was supported by the top talent program of Henan Agricultural University [grant numbers 30501029].

  • Received date 28 June 2022, Accepted date 18 August 2022, RevRecd date 10 August 2022, Publish date 25 August 2022,
    Abstract
  • The pursuit of high-performance is worth considerable effort in catalysis for energy efficiency and environmental sustainability. To develop redox catalysts with superior performance for soot combustion, a series of MnxCoy oxides were synthesized using MgO template substitution. This method greatly improves the preparation and catalytic efficiency and is more in line with the current theme of green catalysts and sustainable development. The resulting Mn1Co2.3 has a strong activation capability of gaseous oxygen due to a high concentration of Co3+ and Mn3+. The Mn doping enhanced the intrinsic activity by prompting oxygen vacancy formation and gaseous oxygen adsorption. The nanosheet morphology with abundant mesoporous significantly increased the solid–solid contact efficiency and improved the adsorption capability of gaseous reactants. The novel design of Mn1Co2.3 oxide enhanced its catalytic performance through a synergistic effect of Mn doping and the porous nanosheet morphology, showing significant potential for the preparation of high-performance soot combustion catalysts.

     

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