Volume 9 Issue 3
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Article Navigation >  Green Energy&Environment  > 2024  >  9(3): 507-515
Ying-Xi Dang, Peng Tan, Bin Hu, Chen Gu, Xiao-Qin Liu, Lin-Bing Sun. Low-energy-consumption temperature swing system for CO2 capture by combining passive radiative cooling and solar heating. Green Energy&Environment, 2024, 9(3): 507-515. doi: 10.1016/j.gee.2022.08.004
Citation: Ying-Xi Dang, Peng Tan, Bin Hu, Chen Gu, Xiao-Qin Liu, Lin-Bing Sun. Low-energy-consumption temperature swing system for CO2 capture by combining passive radiative cooling and solar heating. Green Energy&Environment, 2024, 9(3): 507-515. doi: 10.1016/j.gee.2022.08.004
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Low-energy-consumption temperature swing system for CO2 capture by combining passive radiative cooling and solar heating

doi: 10.1016/j.gee.2022.08.004

  • State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), College of Chemical Engineering, Nanjing Tech University, Nanjing, 211816, China

Funds:

This work was supported by the National Science Fund for Distinguished Young Scholars (22125804) and the National Natural Science Foundation of China (21808110, 22078155, and 21878149).

  • Received date 19 April 2022, Accepted date 08 August 2022, RevRecd date 02 August 2022, Publish date 14 August 2022,
    Abstract
  • Temperature-swing adsorption (TSA) is an effective technique for CO2 capture, but the temperature swing procedure is energy-intensive. Herein, we report a low-energy-consumption system by combining passive radiative cooling and solar heating for the uptake of CO2 on commercial activated carbons (CACs). During adsorption, the adsorbents are coated with a layer of hierarchically porous poly(vinylidene fluoride-co-hexafluoropropene) [P(VdF-HFP)HP], which cools the adsorbents to a low temperature under sunlight through radiative cooling. For desorption, CACs with broad absorption of the solar spectrum are exposed to light irradiation for heating. The heating and cooling processes are completely driven by solar energy. Adsorption tests under mimicked sunlight using the CACs show that the performance of this system is comparable to that of the traditional ones. Furthermore, under real sunlight irradiation, the adsorption capacity of the CACs can be well maintained after multiple cycles. The present work may inspire the development of new temperature swing procedures with little energy consumption.

     

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