Volume 8 Issue 6
Dec.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(6): 1509-1530
Jun-Fan Ding, Yu-Tong Zhang, Rui Xu, Rui Zhang, Ye Xiao, Shuo Zhang, Chen-Xi Bi, Cheng Tang, Rong Xiang, Ho Seok Park, Qiang Zhang, Jia-Qi Huang. Review on lithium metal anodes towards high energy density batteries. Green Energy&Environment, 2023, 8(6): 1509-1530. doi: 10.1016/j.gee.2022.08.002
Citation: Jun-Fan Ding, Yu-Tong Zhang, Rui Xu, Rui Zhang, Ye Xiao, Shuo Zhang, Chen-Xi Bi, Cheng Tang, Rong Xiang, Ho Seok Park, Qiang Zhang, Jia-Qi Huang. Review on lithium metal anodes towards high energy density batteries. Green Energy&Environment, 2023, 8(6): 1509-1530. doi: 10.1016/j.gee.2022.08.002
shu

Review on lithium metal anodes towards high energy density batteries

doi: 10.1016/j.gee.2022.08.002

  • a. School of Materials Science and Engineering, Beijing Institute of Technology, Beijing, 100081, China;

  • b. Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing, 100081, China;

  • c. School of Chemical Engineering and Advanced Materials, The University of Adelaide, Adelaide, SA, 5005 Australia;

  • d. Department of Mechanical Engineering, The University of Tokyo, Tokyo, 113-8656, Japan;

  • e. State Key Laboratory of Fluid Power and Mechatronic Systems, School of Mechanical Engineering, Zhejiang University, Hangzhou, 310027, China;

  • f. School of Chemical Engineering, Sungkyunkwan University, Suwon, 440-746, Republic of Korea;

  • g. Department of Chemical Engineering, Tsinghua University, Beijing, 100084, China

Funds:

This work was supported by National Key Research and Development Program (2021YFB2400300), Beijing Natural Science Foundation (JQ20004), the National Natural Science Foundation of China (22109011, U1801257), and Scientific and Technological Key Project of Shanxi Province (20191102003).

  • Received date 01 June 2022, Accepted date 03 August 2022, RevRecd date 23 July 2022, Publish date 14 August 2022,
    Abstract
  • Lithium metal anode (LMA) is a promising candidate for achieving next-generation high-energy-density batteries due to its ultrahigh theoretical capacity and most negative electrochemical potential. However, the practical application of lithium metal battery (LMB) is largely retarded by the instable interfaces, uncontrolled dendrites, and rapid capacity deterioration. Herein, we present a comprehensive overview towards the working principles and inherent challenges of LMAs. Firstly, we diligently summarize the intrinsic mechanism of Li stripping and plating process. The recent advances in atomic and mesoscale simulations which are crucial in guiding mechanism study and material design are also summarized. Furthermore, the advanced engineering strategies which have been proved effective in protecting LMAs are systematically reviewed, including electrolyte optimization, artificial interface, composite/alloy anodes and so on. Finally, we highlight the current limitations and promising research directions of LMAs. This review sheds new lights on deeply understanding the intrinsic mechanism of LMAs, and calls for more endeavors to realize practical Li metal batteries.

     

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