Volume 8 Issue 6
Dec.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(6): 1596-1618
Jing Xiao, Jia Chen, Juewen Liu, Hirotaka Ihara, Hongdeng Qiu. Synthesis strategies of covalent organic frameworks: An overview from nonconventional heating methods and reaction media. Green Energy&Environment, 2023, 8(6): 1596-1618. doi: 10.1016/j.gee.2022.05.003
Citation: Jing Xiao, Jia Chen, Juewen Liu, Hirotaka Ihara, Hongdeng Qiu. Synthesis strategies of covalent organic frameworks: An overview from nonconventional heating methods and reaction media. Green Energy&Environment, 2023, 8(6): 1596-1618. doi: 10.1016/j.gee.2022.05.003
shu

Synthesis strategies of covalent organic frameworks: An overview from nonconventional heating methods and reaction media

doi: 10.1016/j.gee.2022.05.003

  • a. CAS Key Laboratory of Chemistry of Northwestern Plant Resources and Key Laboratory for Natural Medicine of Gansu Province, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China;

  • b. University of Chinese Academy of Sciences, Beijing 100049, China;

  • c. Department of Chemistry, Waterloo Institute for Nanotechnology, University of Waterloo, Waterloo, Ontario N2L 3G1, Canada;

  • d. Department of Applied Chemistry and Biochemistry, Kumamoto University, 2-39-1 Kurokami, Chuo-ku Kumamoto 860-8555, Japan;

  • e. College of Chemistry, Zhengzhou University, Zhengzhou 450001, China

Funds:

Tech Research Project of Gansu Province (20JR10RA045 and 20JR5RA573). Thanks to Prof. Yi-Tao Long from Nanjing University for his good suggestion.

This work was supported by the National Natural Science Foundation of China (Nos. 21822407 and 22074154), Youth Innovation Promotion Association CAS (2021420) and the Foundation for Sci &

  • Received date 05 March 2022, Accepted date 07 May 2022, RevRecd date 22 April 2022, Publish date 14 May 2022,
    Abstract
  • Covalent organic frameworks (COFs), as an emerging class of porous crystalline materials constructed by covalent links between the building monomers, have gained tremendous attention. Over the past 15 years, COFs have made rapid progress and substantial development in the chemistry and materials fields. However, the synthesis of COFs has been dominated by solvothermal methods for a long time and it usually involves high temperature, high pressure and toxic organic solvents, which created many challenges for environmental considerations. Recently, the exploration of new approaches for facile fabrication of COFs has aroused extensive interest. Hence, in this review, we comprehensively describe the synthetic strategies of COFs from the aspects of nonconventional heating methods and reaction media. In addition, the advantages, limitations and properties of the preparation methods are compared. Finally, we outline the main challenges and development prospects of the synthesis of COFs in the future and propose some possible solutions.

     

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