Volume 8 Issue 4
Aug.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(4): 1006-1042
Yuzhu Chu, Lingxiao Ren, Zhenglin Hu, Chengde Huang, Jiayan Luo. An in-depth understanding of improvement strategies and corresponding characterizations towards Zn anode in aqueous Zn-ions batteries. Green Energy&Environment, 2023, 8(4): 1006-1042. doi: 10.1016/j.gee.2022.04.008
Citation: Yuzhu Chu, Lingxiao Ren, Zhenglin Hu, Chengde Huang, Jiayan Luo. An in-depth understanding of improvement strategies and corresponding characterizations towards Zn anode in aqueous Zn-ions batteries. Green Energy&Environment, 2023, 8(4): 1006-1042. doi: 10.1016/j.gee.2022.04.008
shu

An in-depth understanding of improvement strategies and corresponding characterizations towards Zn anode in aqueous Zn-ions batteries

doi: 10.1016/j.gee.2022.04.008

  • a. Key Laboratory for Green Chemical Technology of Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Tianjin, 300072, China;

  • b. Key Laboratory of Materials Processing and Mold (Zhengzhou University), Ministry of Education, Zhengzhou, 450002, China;

  • c. Shanghai Key Lab of Advanced High-Temperature Materials and Precision Forming, School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai, 200240, China

Funds:

This work was supported by the National Natural Science Foundation of China (Grant Nos. 51872196).

  • Received date 09 March 2022, Accepted date 28 April 2022, RevRecd date 28 April 2022, Publish date 05 May 2022,
    Abstract
  • Combining the unique advantages of aqueous electrolytes and metallic Zn anode, rechargeable aqueous Zn-ion batteries (ZIBs) are of great promise for large-scale energy storage applications due to their inherent high safety, low cost, and environmental friendliness. As the essential component of ZIBs, Zn metal anode suffers from severe dendrite formation and inevitable side reactions (e.g. corrosion and hydrogen evolution) in aqueous electrolytes, which leads to low Coulombic efficiency and inferior cycling stability, impeding their large-scale applications. To be compatible with satisfactory aqueous ZIBs, Zn anode has been modified from various perspectives and focus areas. Herein, based on their intrinsic characteristics, we review the related improvement strategies for Zn anode, including interphase, substrate, and bulk design, so as to achieve an in-depth understanding of Zn anode optimization. Furthermore, the timely summary of characterization methods for Zn anodes are also performed for the first time, from both thermodynamic and kinetics perspectives, which is particularly helpful for beginners to understand the complicated characterizations and employ suitable methods. Finally, certain noteworthy points are put forward for subsequent investigation of aqueous ZIBs. It is expected that this review will enlighten researchers to explore more efficient optimization strategies for Zn anode in aqueous electrolytes.

     

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