Volume 9 Issue 4
Apr.  2024
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Article Navigation >  Green Energy&Environment  > 2024  >  9(4): 684-694
Guangfu Qian, Wei Chen, Jinli Chen, Li Yong Gan, Tianqi Yu, Miaojing Pan, Xiaoyan Zhuo, Shibin Yin. Pyridinic-N doping carbon layers coupled with tensile strain of FeNi alloy for activating water and urea oxidation. Green Energy&Environment, 2024, 9(4): 684-694. doi: 10.1016/j.gee.2022.04.006
Citation: Guangfu Qian, Wei Chen, Jinli Chen, Li Yong Gan, Tianqi Yu, Miaojing Pan, Xiaoyan Zhuo, Shibin Yin. Pyridinic-N doping carbon layers coupled with tensile strain of FeNi alloy for activating water and urea oxidation. Green Energy&Environment, 2024, 9(4): 684-694. doi: 10.1016/j.gee.2022.04.006
shu

Pyridinic-N doping carbon layers coupled with tensile strain of FeNi alloy for activating water and urea oxidation

doi: 10.1016/j.gee.2022.04.006

  • a. Guangxi Key Laboratory of Electrochemical Energy Materials, College of Chemistry and Chemical Engineering, State Key Laboratory of Processing for Non-Ferrous Metal and Featured Materials, Guangxi University, 100 Daxue Road, Nanning, 530004, China;

  • b. Institute for Structure and Function and Department of Physics, Chongqing University, Chongqing, 400030, China

Funds:

This work is supported by the National Natural Science Foundation of China (21872040, 22162004), the Excellent Scholars and Innovation Team of Guangxi Universities, the Innovation Project of Guangxi Graduate Education (YCBZ2022038), and the High-performance Computing Platform of Guangxi University.

  • Received date 14 March 2022, Accepted date 26 April 2022, RevRecd date 18 April 2022, Publish date 10 May 2022,
    Abstract
  • Exploitation of oxygen evolution reaction (OER) and urea oxidation reaction (UOR) catalysts with high activity and stability at large current density is a major challenge for energy-saving H2 production in water electrolysis. Herein, we use the pyridinic-N doping carbon layers coupled with tensile strain of FeNi alloy activated by NiFe2O4 (FeNi/NiFe2O4@NC) for efficiently increasing the performance of water and urea oxidation. Due to the tensile strain effect on FeNi/NiFe2O4@NC, it provides a favorable modulation on the electronic properties of the active center, thus enabling amazing OER (η100 = 196 mV) and UOR (E10 = 1.32 V) intrinsic activity. Besides, the carbon-coated layers can be used as armor to prevent FeNi alloy from being corroded by the electrolyte for enhancing the OER/UOR stability at large current density, showing high industrial practicability. This work thus provides a simple way to prepare high-efficiency catalyst for activating water and urea oxidation.

     

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