Volume 8 Issue 6
Dec.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(6): 1711-1718
Gongxun Zhai, Qianqian Wang, Fuyao Liu, Zexu Hu, Chao Jia, Dengxin Li, Hengxue Xiang, Meifang Zhu. One-step floating conversion of biomass into highly graphitized and continuous carbon nanotube yarns. Green Energy&Environment, 2023, 8(6): 1711-1718. doi: 10.1016/j.gee.2022.04.002
Citation: Gongxun Zhai, Qianqian Wang, Fuyao Liu, Zexu Hu, Chao Jia, Dengxin Li, Hengxue Xiang, Meifang Zhu. One-step floating conversion of biomass into highly graphitized and continuous carbon nanotube yarns. Green Energy&Environment, 2023, 8(6): 1711-1718. doi: 10.1016/j.gee.2022.04.002
shu

One-step floating conversion of biomass into highly graphitized and continuous carbon nanotube yarns

doi: 10.1016/j.gee.2022.04.002

  • State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, China

Funds:

The authors gratefully acknowledge the support from the Science and Technology Commission of Shanghai Municipality (20JC1414900), the Joint Funds of the National Natural Science Foundation of China (U20A20257), the Program of Shanghai Academic/Technology Research Leader (20XD1433700), and the International Cooperation Fund of the Science and Technology Commission of Shanghai Municipality (20520740800).

  • Received date 16 February 2022, Accepted date 20 April 2022, RevRecd date 19 April 2022, Publish date 26 April 2022,
    Abstract
  • The rapid growth of the demand for carbon nanotubes (CNTs) has greatly promoted their large-scale synthesis and development. However, the continuous production of CNT fibers by floating catalyst chemical vapor deposition (FCCVD) requires a large amount of non-renewable carbon sources. Here, the continuous production of highly graphitized CNT yarns from biomass tannic acid (TA) is reported. The chelation of TA and catalyst promotes the rapid cracking of biomass into carbon source gas, and the pyrolysis cracking produces the reducing gas, which solves the problems of the continuous production of CNT yarns using biomass. Through simple twisting, the mechanical strength of CNT yarn can reach 886 ±46 MPa, and the electrical conductivity and graphitization (IG/ID) can reach 2×105 S m-1 and 6.3, respectively. This work presents a promising solution for the continuous preparation of CNT yarns based on green raw material.

     

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