Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO<sub>2</sub>

Xin Yu; Tingke Jin; Huiqiang Wang; Guoqing Zhang; Wenlong Jia; Lincai Peng; Yong Sun; Xing Tang; Xianhai Zeng; Shuliang Yang; Zheng Li; Feng Xu; Lu Lin

doi:10.1016/j.gee.2022.03.016

Volume 8 Issue 6

Dec. 2023

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Article Navigation > Green Energy&Environment > 2023 > 8(6): 1683-1692

Xin Yu, Tingke Jin, Huiqiang Wang, Guoqing Zhang, Wenlong Jia, Lincai Peng, Yong Sun, Xing Tang, Xianhai Zeng, Shuliang Yang, Zheng Li, Feng Xu, Lu Lin. Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO2. Green Energy&Environment, 2023, 8(6): 1683-1692. doi: 10.1016/j.gee.2022.03.016

Citation:

Xin Yu, Tingke Jin, Huiqiang Wang, Guoqing Zhang, Wenlong Jia, Lincai Peng, Yong Sun, Xing Tang, Xianhai Zeng, Shuliang Yang, Zheng Li, Feng Xu, Lu Lin. Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO₂. Green Energy&Environment, 2023, 8(6): 1683-1692. doi: 10.1016/j.gee.2022.03.016

Citation:

Xin Yu, Tingke Jin, Huiqiang Wang, Guoqing Zhang, Wenlong Jia, Lincai Peng, Yong Sun, Xing Tang, Xianhai Zeng, Shuliang Yang, Zheng Li, Feng Xu, Lu Lin. Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO₂. Green Energy&Environment, 2023, 8(6): 1683-1692. doi: 10.1016/j.gee.2022.03.016

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Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO₂

doi: 10.1016/j.gee.2022.03.016

Xin Yu^a,
Tingke Jin^b,
Huiqiang Wang^a,
Guoqing Zhang^a,
Wenlong Jia^a,
Lincai Peng^c,
Yong Sun^{a,d,e
,
,},
Xing Tang^a,d,e,
Xianhai Zeng^a,d,e,
Shuliang Yang^a,d,e,
Zheng Li^a,d,e,
Feng Xu^f,
Lu Lin^a,d,e

Abstract

Abstract

A cost-effective and sustainable noble-metal free catalyst system based on ubiquitously available Mn-Cu bimetallic oxides was served as efficient catalysts for furfural selective oxidation to furancarboxylic acid (FA). Interestingly, Mn₂Cu₁O_x exhibited an excellent furfural conversion of 99% with quantitative selectivity toward FA. Especially, we demonstrate the significant weakening of the Mn-O bonds with the incorporation of CuO into the Mn-Cu oxides, resulting in an improved O_L reactivity of Mn₂Cu₁O_x, which brings about a higher catalytic activity for furfural oxidation. More importantly, Mn₂Cu₁O_x could exhibit Y_FA>90% over 5 cycles of reusability test. Through this study, the relationship between the morphology, surface chemistry, and catalytic activity of Mn-Cu bimetallic oxides are elucidated, providing a simple and environmentally friendly catalytic strategy and scientific basis for the development of Mn-Cu bimetallic oxides bioderived molecular aerobic oxidation materials.
- Furfural,
- Mn-Cu bimetallic oxides,
- Oxidation,
- Lattice oxygen,
- Furancarboxylic acid

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References

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Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO₂

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Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO2

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Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO₂