Volume 8 Issue 6
Dec.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(6): 1683-1692
Xin Yu, Tingke Jin, Huiqiang Wang, Guoqing Zhang, Wenlong Jia, Lincai Peng, Yong Sun, Xing Tang, Xianhai Zeng, Shuliang Yang, Zheng Li, Feng Xu, Lu Lin. Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO2. Green Energy&Environment, 2023, 8(6): 1683-1692. doi: 10.1016/j.gee.2022.03.016
Citation: Xin Yu, Tingke Jin, Huiqiang Wang, Guoqing Zhang, Wenlong Jia, Lincai Peng, Yong Sun, Xing Tang, Xianhai Zeng, Shuliang Yang, Zheng Li, Feng Xu, Lu Lin. Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO2. Green Energy&Environment, 2023, 8(6): 1683-1692. doi: 10.1016/j.gee.2022.03.016
shu

Heterogeneously-catalyzed aerobic oxidation of furfural to furancarboxylic acid with CuO-Promoted MnO2

doi: 10.1016/j.gee.2022.03.016

  • a. College of Energy, Xiamen University, Xiamen, 361102, China;

  • b. Institute of Geology, Xibu Drilling Engineering Company Limited, China National Petroleum Corporation, Xinjiang, 834000, China;

  • c. BiomassChem Group, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming, Yunnan, 650500, China;

  • d. Fujian Engineering and Research Center of Clean and High-valued Technologies for Biomass, China;

  • e. Xiamen Key Laboratory of High-valued Utilization of Biomass, Xiamen University, Xiamen, 361102, China;

  • f. Beijing Forestry Univ, Inst Biomass Chem & Technol, Beijing, 100083, China

Funds:

This work was supported by the National Natural Science Fund of China (Nos. 21978246 and 21776234).

  • Received date 24 February 2022, Accepted date 31 March 2022, RevRecd date 28 March 2022, Publish date 06 April 2022,
    Abstract
  • A cost-effective and sustainable noble-metal free catalyst system based on ubiquitously available Mn-Cu bimetallic oxides was served as efficient catalysts for furfural selective oxidation to furancarboxylic acid (FA). Interestingly, Mn2Cu1Ox exhibited an excellent furfural conversion of 99% with quantitative selectivity toward FA. Especially, we demonstrate the significant weakening of the Mn-O bonds with the incorporation of CuO into the Mn-Cu oxides, resulting in an improved OL reactivity of Mn2Cu1Ox, which brings about a higher catalytic activity for furfural oxidation. More importantly, Mn2Cu1Ox could exhibit YFA>90% over 5 cycles of reusability test. Through this study, the relationship between the morphology, surface chemistry, and catalytic activity of Mn-Cu bimetallic oxides are elucidated, providing a simple and environmentally friendly catalytic strategy and scientific basis for the development of Mn-Cu bimetallic oxides bioderived molecular aerobic oxidation materials.

     

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