Volume 8 Issue 6
Dec.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(6): 1673-1682
Chizhou Wang, Shaodi Wu, Ning Zhang, Zhaoli Jiang, Xianglin Hou, Long Huang, Tiansheng Deng. Efficient oil-water separation by novel biodegradable all cellulose composite filter paper. Green Energy&Environment, 2023, 8(6): 1673-1682. doi: 10.1016/j.gee.2022.03.013
Citation: Chizhou Wang, Shaodi Wu, Ning Zhang, Zhaoli Jiang, Xianglin Hou, Long Huang, Tiansheng Deng. Efficient oil-water separation by novel biodegradable all cellulose composite filter paper. Green Energy&Environment, 2023, 8(6): 1673-1682. doi: 10.1016/j.gee.2022.03.013
shu

Efficient oil-water separation by novel biodegradable all cellulose composite filter paper

doi: 10.1016/j.gee.2022.03.013

  • a. Shanxi Engineering Research Center of Biorefinery, Institute of Coal Chemistry, Chinese Academy of Sciences, 27 South Taoyuan Road, Taiyuan, 030001, China;

  • b. Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049, China;

  • c. Key Laboratory of China Research Institute of Daily Chemistry Co., Ltd., Sinolight Corporation, Taiyuan, 030001, China;

  • d. CAS Key Laboratory of Carbon Materials, Institute of Coal Chemistry, Chinese Academy of Sciences, 27 South Taoyuan Road, Taiyuan, 030001, China;

  • e. Beijing Key Laboratory of Fuels Cleaning and Advanced Catalytic Emission Reduction Technology, Beijing Institute of Petrochemical Technology, Beijing, 102617, China

Funds:

The authors gratefully acknowledge the financial support from the National Key R&

D Program of China (no. 2018YFB1501602), Science Foundation of Shanxi Province, China (Grant no. 201901D111006ZD), Fund for Shanxi “1331 project”, and Shanxi Province Platform Base and Talent Special Fund (no. 201705D211023).

  • Received date 17 January 2022, Accepted date 29 March 2022, RevRecd date 17 March 2022, Publish date 06 April 2022,
    Abstract
  • Industrial production and domestic discharge produce a large amount of oily wastewater, which seriously affects the stability of the ecological environment. Membrane separation technology provides another path to treating oily wastewater. And appropriate surface modification of the membrane helps to achieve high efficiency of treating oily wastewater. With green, economy and stability been more concerned. The focal research reports a completely biodegradable all cellulose composite filter paper (ACCFP) composed of I-cellulose macrofibers and II-cellulose matrix. It is a simple one-step impregnation method to adjust the surface microstructure of the pristine filter paper (PFP), and it does not involve with chemical reaction. The pre-wetted ACCFP consist of II-cellulose hydrogel and I-cellulose reinforcement in the process of oil-water separation. This layer of hydrogel is the fundamental to underwater superoleophobicity, which determines their eligibility for applications of efficient oil-water mixture or oil-in-water (oil/water) emulsion separation. The separation efficiency of oil-water mixture and oil/water emulsion exceed 95% and 99.9%, respectively. In addition, excellent mechanical properties of ACCFP in dry and wet conditions ensure its stability in service and prolong service life in applications. The focal study provides a new method for high-performance oil-water separation and it is more in line with sustainable chemistry.

     

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