Volume 8 Issue 6
Dec.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(6): 1644-1653
Pei Xiong, Peng He, Yixin Qu, Liguo Wang, Yan Cao, Shuang Xu, Jiaqiang Chen, Muhammad Ammar, Huiquan Li. The adsorption properties of NaY zeolite for separation of ethylene glycol and 1,2-butanediol: Experiment and molecular modelling. Green Energy&Environment, 2021, 6(1): 102-113. doi: 10.1016/j.gee.2019.12.006
Citation: Qiuyan Jin, Liping Xiao, Weidong He, Hao Cui, Chengxin Wang. Self-supported metal (Fe, Co, Ni)-embedded nitrogen-doping carbon nanorod framework as trifunctional electrode for flexible Zn-air batteries and switchable water electrolysis. Green Energy&Environment, 2023, 8(6): 1644-1653. doi: 10.1016/j.gee.2022.03.008
shu

Self-supported metal (Fe, Co, Ni)-embedded nitrogen-doping carbon nanorod framework as trifunctional electrode for flexible Zn-air batteries and switchable water electrolysis

doi: 10.1016/j.gee.2022.03.008

  • a. State Key Laboratory of Optoelectronic Materials and Technologies, School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou, 510275, China;

  • b. The Key Laboratory of Low-Carbon Chemistry & Energy Conservation of Guangdong Province, Sun Yat-sen University, Guangzhou, 510275, China

Funds:

This work was financially supported by the National Natural Science Foundation of China (Grants Nos. 51972349, U1801255 and 91963210).

  • Received date 23 December 2021, Accepted date 22 March 2022, RevRecd date 08 March 2022, Publish date 30 March 2022,
    Abstract
  • To meet the practical demand of wearable/portable electronics, developing high-efficiency and durable multifunctional catalyst and in-situ assembling catalysts into electrodes with flexible features are urgently needed but challenging. Herein, we report a simple route to fabricate bendable multifunctional electrodes by in-situ carbonization of metal ion absorbed polyaniline precursor. Alloy nanoparticles encapsulated in graphite layer are uniformly distributed in the N-doping carbon nanorod skeleton. Profiting from the favorable free-standing structure and the cooperative effect of metallic nanoparticles, graphitic layer and N doped-carbon architecture, the trifunctional electrodes exhibit prominent activities and stability toward HER, OER and ORR. Notably, due to the protection of carbon layer, the electrocatalysts show the reversible catalytic HER/OER properties. The overall water splitting device can continuously work for 12 h under frequent exchanges of cathode and anode. Importantly, the bendable metal air batteries fabricated by self-supported electrode not only displays the outstanding battery performance, achieving a decent peak power density (125 mW cm-2) and exhibiting favorable charge-discharge durability of 22 h, but also holds superb flexible stability. Specially, a lightweight self-driven water splitting unit is demonstrated with stable hydrogen production.

     

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