Volume 8 Issue 5
Oct.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(5): 1459-1468
Pan Wu, Xuan Wu, Yida Wang, Jingyuan Zhao, Haolan Xu, Gary Owens. Boosting extraction of Pb in contaminated soil via interfacial solar evaporation of multifunctional sponge. Green Energy&Environment, 2023, 8(5): 1459-1468. doi: 10.1016/j.gee.2022.03.002
Citation: Pan Wu, Xuan Wu, Yida Wang, Jingyuan Zhao, Haolan Xu, Gary Owens. Boosting extraction of Pb in contaminated soil via interfacial solar evaporation of multifunctional sponge. Green Energy&Environment, 2023, 8(5): 1459-1468. doi: 10.1016/j.gee.2022.03.002
shu

Boosting extraction of Pb in contaminated soil via interfacial solar evaporation of multifunctional sponge

doi: 10.1016/j.gee.2022.03.002

  • Future Industries Institute, UniSA STEM, University of South Australia, Mawson Lakes Campus, SA 5095, Australia

Funds:

H. Xu acknowledges the financial support from the Australian Research Council (FT190100485, DP220100583). P.W. acknowledge financial support from the China Scholarship Council for primary scholarships and from the Future Industries Institute for top up scholarships. All authors acknowledge the use of Microscopy Australia facilities located at the University of South Australia, infrastructure co-funded by the University of South Australia, the South Australian State Government, and the Australian Federal Government's National Collaborative Research Infrastructure Strategy (NCRIS) scheme.

  • Received date 09 December 2021, Accepted date 03 March 2022, RevRecd date 20 February 2022, Publish date 09 March 2022,
    Abstract
  • Interfacial solar water evaporation is a reliable way to accelerate water evaporation and contaminant remediation. Embracing the recent advance in photothermal technology, a functional sponge was prepared by coating a sodium alginate (SA) impregnated sponge with a surface layer of reduced graphene oxide (rGO) to act as a photothermal conversion medium and then subsequently evaluated for its ability to enhance Pb extraction from contaminated soil driven by interfacial solar evaporation. The SA loaded sponge had a Pb adsorption capacity of 107.4 mg g−1. Coating the top surface of the SA sponge with rGO increased water evaporation performance to 1.81 kg m−2 h−1 in soil media under one sun illumination and with a wind velocity of 2 m s−1. Over 12 continuous days of indoor evaporation testing, the Pb extraction efficiency was increased by 22.0% under 1 sun illumination relative to that observed without illumination. Subsequently, Pb extraction was further improved by 48.9% under outdoor evaporation conditions compared to indoor conditions. Overall, this initial work shows the significant potential of interfacial solar evaporation technologies for Pb contaminated soil remediation, which should also be applicable to a variety of other environmental contaminants.

     

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