Volume 8 Issue 5
Oct.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(5): 1450-1458
Jingyi Wang, Jiajia Huang, Siyu Zhao, Ivan P. Parkin, Zhihong Tian, Feili Lai, Tianxi Liu, Guanjie He. Mo/Fe bimetallic pyrophosphates derived from Prussian blue analogues for rapid electrocatalytic oxygen evolution. Green Energy&Environment, 2023, 8(5): 1450-1458. doi: 10.1016/j.gee.2022.02.014
Citation: Jingyi Wang, Jiajia Huang, Siyu Zhao, Ivan P. Parkin, Zhihong Tian, Feili Lai, Tianxi Liu, Guanjie He. Mo/Fe bimetallic pyrophosphates derived from Prussian blue analogues for rapid electrocatalytic oxygen evolution. Green Energy&Environment, 2023, 8(5): 1450-1458. doi: 10.1016/j.gee.2022.02.014
shu

Mo/Fe bimetallic pyrophosphates derived from Prussian blue analogues for rapid electrocatalytic oxygen evolution

doi: 10.1016/j.gee.2022.02.014

  • a. School of Chemical Engineering, Zhengzhou University, Zhengzhou, 450001, China;

  • b. Department of Chemistry, University College London, London, WC1H 0AJ, UK;

  • c. School of Chemistry, University of Lincoln, Joseph Banks Laboratories, Green Lane, Lincoln, LN6 7DL, UK;

  • d. Henan University, Jinming Avenue, Kaifeng, 475001, China;

  • e. Department of Chemistry, KU Leuven, Celestijnenlaan 200F, Leuven, 3001, Belgium;

  • f. Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, International Joint Research Laboratory for Nano Energy Composites, Jiangnan University, Wuxi, 214122, China

Funds:

This work was supported by National Natural Science Foundation of China (No. 51873198), the Engineering and Physical Sciences Research Council (EPSRC, EP/V027433/1), and the Royal Society (RGS∖R1∖211080).

  • Received date 16 January 2022, Accepted date 27 February 2022, RevRecd date 20 February 2022, Publish date 03 March 2022,
    Abstract
  • Efficient and stable oxygen evolution electrocatalysts are indispensable for industrial applications of water splitting and hydrogen production. Herein, a simple and practical method was applied to fabricate (Mo, Fe)P2O7@NF electrocatalyst by directly growing Mo/Fe bimetallic pyrophosphate derived from Prussian blue analogues on three-dimensional porous current collector. In alkaline media, the developed material possesses good hydrophilic features and exhibits best-in-class oxygen evolution reaction (OER) performances. Surprisingly, the (Mo, Fe)P2O7@NF only requires overpotentials of 250 and 290 mV to deliver 100 and 600 mA cm−2 in 1 mol L−1 KOH, respectively. Furthermore, the (Mo, Fe)P2O7@NF shows outstanding performances in alkaline salty water and 1 mol L−1 high purity KOH. A worthwhile pathway is provided to combine bimetallic pyrophosphate with commercial Ni foam to form robust electrocatalysts for stable electrocatalytic OER, which has a positive impact on both hydrogen energy application and environmental restoration.

     

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