Volume 8 Issue 2
Apr.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(2): 579-588
Quanzhou Du, Yuhua Zhao, Yujuan Chen, Jianming Liu, Huanhuan Li, Guangyue Bai, Kelei Zhuo, Jianji Wang. Nitrogen-doped porous carbon nanosheets as both anode and cathode for advanced potassium-ion hybrid capacitors. Green Energy&Environment, 2023, 8(2): 579-588. doi: 10.1016/j.gee.2022.02.013
Citation: Quanzhou Du, Yuhua Zhao, Yujuan Chen, Jianming Liu, Huanhuan Li, Guangyue Bai, Kelei Zhuo, Jianji Wang. Nitrogen-doped porous carbon nanosheets as both anode and cathode for advanced potassium-ion hybrid capacitors. Green Energy&Environment, 2023, 8(2): 579-588. doi: 10.1016/j.gee.2022.02.013
shu

Nitrogen-doped porous carbon nanosheets as both anode and cathode for advanced potassium-ion hybrid capacitors

doi: 10.1016/j.gee.2022.02.013

  • Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals, Key Laboratory of Green Chemical Media and Reactions, Ministry of Education, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang, Henan, 453007, China

Funds:

This work was financially supported by the National Natural Science Foundation of China (Nos. 21873026, 21573061, 21773059).

  • Received date 25 December 2021, Accepted date 23 February 2022, RevRecd date 23 February 2022, Publish date 01 March 2022,
    Abstract
  • Potassium-ion hybrid capacitors (PIHCs) as a burgeoning research hotspot are an ideal replacement for lithium-ion hybrid capacitors (LIHCs). Here, we report nitrogen-doped porous carbon nanosheets (NPCNs) with enlarged interlayer spacing, abundant defects, and favorable mesoporous structures. The structural changes of NPCNs in potassiation and depotassiation processes are analyzed by using Raman spectroscopy and transmission electron microscopy. Due to the unique structure of NPCNs, the PIHC device assembled using NPCNs as both the anode and cathode material (double-functional self-matching material) exhibits a superior energy density of 128 Wh kg-1 with a capacity retention of 90.8% after 9000 cycles. This research can promote the development of double-functional self-matching materials for hybrid energy storage devices with ultra-high performance.

     

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