Volume 8 Issue 5
Oct.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(5): 1429-1436
Yuxin Gao, Jiang Zhou, Liping Qin, Zhenming Xu, Zhexuan Liu, Liangbing Wang, Xinxin Cao, Guozhao Fang, Shuquan Liang. Crystal plane induced in-situ electrochemical activation of manganese-based cathode enable long-term aqueous zinc-ion batteries. Green Energy&Environment, 2023, 8(5): 1429-1436. doi: 10.1016/j.gee.2022.02.009
Citation: Yuxin Gao, Jiang Zhou, Liping Qin, Zhenming Xu, Zhexuan Liu, Liangbing Wang, Xinxin Cao, Guozhao Fang, Shuquan Liang. Crystal plane induced in-situ electrochemical activation of manganese-based cathode enable long-term aqueous zinc-ion batteries. Green Energy&Environment, 2023, 8(5): 1429-1436. doi: 10.1016/j.gee.2022.02.009
shu

Crystal plane induced in-situ electrochemical activation of manganese-based cathode enable long-term aqueous zinc-ion batteries

doi: 10.1016/j.gee.2022.02.009

  • a. School of Materials Science and Engineering, Central South University, Changsha, 410083, Hunan, China;

  • b. Graduate Department, Guangxi University of Science and Technology, Liuzhou, 545006, Guangxi, China;

  • c. College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, Jiangsu, China;

  • d. Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province, Central South University, Changsha, 410083, Hunan, China

Funds:

This work was supported by the National Natural Science Foundation of China (Grant Nos. 51932011 and 52072411). Science and technology innovation Program of Hunan Province (Grant no. 2021RC3001). Natural Science Foundation of Hunan Province (Grant no. 2021JJ20060, 2018RS3019 and 2019JJ30033).

  • Received date 01 December 2021, Accepted date 15 February 2022, RevRecd date 09 February 2022, Publish date 22 February 2022,
    Abstract
  • Rapid capacity decay and sluggish reaction kinetics are major barriers hindering the applications of manganese-based cathode materials for aqueous zinc-ion batteries. Herein, the effects of crystal plane on the in-situ transformation behavior and electrochemical performance of manganese-based cathode is discussed. A comprehensive discussion manifests that the exposed (100) crystal plane is beneficial to the phase transformation from tunnel-structured MnO2 to layer-structured ZnMn3O7·3H2O, which plays a critical role for the high reactivity, high capacity, fast diffusion kinetics and long cycling stability. Additionally, a two-stage zinc storage mechanism can be demonstrated, involving continuous activation reaction and phase transition reaction. As expected, it exhibits a high capacity of 275 mAh g−1 at 100 mA g−1, a superior durability over 1000 cycles and good rate capability. This study may open new windows toward developing advanced cathodes for ZIBs, and facilitate the applications of ZIBs in large-scale energy storage system.

     

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