Volume 8 Issue 5
Oct.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(5): 1389-1397
Wei-Shi Sun, Ming-Jie Yin, Wen-Hai Zhang, Shuo Li, Naixin Wang, Quan-Fu An. Tailor-made microstructures lead to high-performance robust PEO membrane for CO2 capture via green fabrication technique. Green Energy&Environment, 2023, 8(5): 1389-1397. doi: 10.1016/j.gee.2022.01.016
Citation: Wei-Shi Sun, Ming-Jie Yin, Wen-Hai Zhang, Shuo Li, Naixin Wang, Quan-Fu An. Tailor-made microstructures lead to high-performance robust PEO membrane for CO2 capture via green fabrication technique. Green Energy&Environment, 2023, 8(5): 1389-1397. doi: 10.1016/j.gee.2022.01.016
shu

Tailor-made microstructures lead to high-performance robust PEO membrane for CO2 capture via green fabrication technique

doi: 10.1016/j.gee.2022.01.016

  • Beijing Key Laboratory for Green Catalysis and Separation, Department of Environmental and Chemical Engineering, Beijing University of Technology, Beijing, 100124, China

Funds:

This research was financially supported by National Natural Science Foundation of China (No. 22125801, 21975005, 21878004) and Cooperative Research Project of BJUT-NTUT (No. 110-03).

  • Received date 07 December 2021, Accepted date 28 January 2022, RevRecd date 18 January 2022, Publish date 09 February 2022,
    Abstract
  • Emerging excessive greenhouse gas emissions pose great threats to the ecosystem, which thus requires efficient CO2 capture to mitigate the disastrous issue. In this report, large molecular size bisphenol A ethoxylate diacrylate (BPA) was employed to crosslink poly (ethylene glycol) methyl ether acrylate (PEGMEA) via the green and rapid UV polymerization strategy. The microstructure of such-prepared membrane could be conveniently tailored by tuning the ratio of the two prepolymers, aiming at obtaining the optimized microstructures with suitable mesh size and PEO sol content, which was approved by a novel low-field nuclear magnetic resonance technique. The optimum membrane overcomes the trade-off challenge: dense microstructures lower the gas permeability while loose microstructures lower high-pressure-resistance capacity, realizing a high CO2 permeability of 1711 Barrer and 100-h long-term running stability under 15 atm. The proposed membrane fabrication approach, hence, opens a novel gate for developing high-performance robust membranes for CO2 capture.

     

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