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Haifang Shen, Hao Li, Zhensheng Yang, Chunli Li. Magic of hydrogen spillover: Understanding and application. Green Energy&Environment, 2022, 7(6): 1161-1198. doi: 10.1016/j.gee.2022.01.013
Citation: Haifang Shen, Hao Li, Zhensheng Yang, Chunli Li. Magic of hydrogen spillover: Understanding and application. Green Energy&Environment, 2022, 7(6): 1161-1198. doi: 10.1016/j.gee.2022.01.013
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Magic of hydrogen spillover: Understanding and application

doi: 10.1016/j.gee.2022.01.013

  • National-Local Joint Engineering Laboratory for Energy Conservation in Chemical Process Integration and Resources Utilization, Tianjin Key Laboratory of Chemical Process Safety, School of Chemical Engineering and Technology, Hebei University of Technology, 8 Guangrong Road, Tianjin, 300130, China

Funds:

Financial support from the National Natural Science Foundation of China (22108056) and the Scientific Research Projects of Hebei Education Department (QN2019050) and the National Natural Science Foundation of Hebei Province (B2020202004) are gratefully acknowledged. I would also like to thank Professor Sun Zhuohua of Beijing Forestry University for his guidance in writing the paper.

  • Received date 22 October 2021, Accepted date 27 January 2022, RevRecd date 15 January 2022, Publish date 03 February 2022,
    Abstract
  • The hydrogen spillover effect (HSPE) plays an important role in heterogeneous catalysis and hydrogen storage as an interfacial phenomenon, which facilitates the improvement of hydrogen storage properties of porous nanomaterials and indirectly or directly affects the reaction performance of multiphase catalytic reactions. The setting-up of the word “hydrogen spillover” opened up a new area to gain insight into the dynamic behavior of migrating hydrogen atoms on a catalyst surface. However, a comprehensive understanding of the HSPE is still lacking. Today, the development of advanced characterization techniques provides increasingly valuable information to further our understanding of the HSPE. Based on these considerations, in this review, we hope to provide some answers to the question “What is hydrogen spillover and how do we recognize it?”. To do this, we will rely on advanced characterization techniques as well as experimental and theoretical studies. Then, we discuss in detail the influences of the HSPE on hydrogen storage performance and the important catalytic effects of the HSPE in catalysis. These effects will be reviewed by looking through the catalytic results obtained in many reactions in thermal catalysis, electrocatalysis, and photocatalysis. Furthermore, based on the application potential of hydrogen spillover, we present some preliminary research proposals and discuss the opportunities and challenges that remain to be faced in this research area.

     

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