Volume 8 Issue 2
Apr.  2023
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Article Navigation >  Green Energy&Environment  > 2023  >  8(2): 360-382
Yaqi Cao, Wenchao Peng, Yang Li, Fengbao Zhang, Yuanzhi Zhu, Xiaobin Fan. Atomically dispersed metal sites in COF-based nanomaterials for electrochemical energy conversion. Green Energy&Environment, 2023, 8(2): 360-382. doi: 10.1016/j.gee.2021.11.005
Citation: Yaqi Cao, Wenchao Peng, Yang Li, Fengbao Zhang, Yuanzhi Zhu, Xiaobin Fan. Atomically dispersed metal sites in COF-based nanomaterials for electrochemical energy conversion. Green Energy&Environment, 2023, 8(2): 360-382. doi: 10.1016/j.gee.2021.11.005
shu

Atomically dispersed metal sites in COF-based nanomaterials for electrochemical energy conversion

doi: 10.1016/j.gee.2021.11.005

  • a. State Key Laboratory of Chemical Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin, 300350, China;

  • b. Yunnan Provincial Key Laboratory of Energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming, 650500, China

Funds:

This work was supported by the National Natural Science Funds (No. 21878226) and Innovative Research Group Project of the National Natural Science Foundation of China (No. 22121004).

  • Received date 03 September 2021, Accepted date 10 November 2021, RevRecd date 04 November 2021, Available online 20 March 2023, Publish date 31 December 2021,
    Abstract
  • Atomically dispersed metal sites (ADMSs) play key roles in electrochemical energy conversion. The covalent organic frameworks (COFs) enable the precise control of the chemical compositions and structures at the molecular level, making them ideal substrates for supporting ADMSs. In this review, we systematically summarize the recent progress on the design and synthesis of ADMSs in COFs, including embedding molecular catalysts into COFs, immobilizing ADMSs on heteroatom-containing COFs, and preparing COF-derived carbon materials through pyrolysis. The electrocatalytic performance of the resulting catalysts is presented for various electrochemical reactions, involving oxygen reduction reaction (ORR), carbon dioxide reduction reaction (CO2RR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER), and nitrogen reduction reaction (NRR). The modulation strategies of AMDSs in COFs for enhanced activity, selectivity, and stability are highlighted, together with a perspective of the current challenges and the future opportunities in this field.

     

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