Volume 7 Issue 5
Oct.  2022
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Article Navigation >  Green Energy&Environment  > 2022  >  7(5): 900-932
Huai Liu, Xing Tang, Xianhai Zeng, Yong Sun, Xixian Ke, Tianyuan Li, Jiaren Zhang, Lu Lin. Catalyst design strategy toward the efficient heterogeneously-catalyzed selective oxidation of 5-hydroxymethylfurfural. Green Energy&Environment, 2022, 7(5): 900-932. doi: 10.1016/j.gee.2021.10.004
Citation: Huai Liu, Xing Tang, Xianhai Zeng, Yong Sun, Xixian Ke, Tianyuan Li, Jiaren Zhang, Lu Lin. Catalyst design strategy toward the efficient heterogeneously-catalyzed selective oxidation of 5-hydroxymethylfurfural. Green Energy&Environment, 2022, 7(5): 900-932. doi: 10.1016/j.gee.2021.10.004
shu

Catalyst design strategy toward the efficient heterogeneously-catalyzed selective oxidation of 5-hydroxymethylfurfural

doi: 10.1016/j.gee.2021.10.004

  • a BiomassChem Group, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming, 650500, China;

  • b Xiamen Key Laboratory of Clean and High-valued Utilization for Biomass, College of Energy, Xiamen University, Xiang'an South Road, Xiamen, 361102, China;

  • c Fujian Engineering and Research Center of Clean and High-valued Technologies for Biomass, Xiamen University, Xiang'an South Road, Xiamen, 361005, China;

  • d Key Lab for Sport Shoes Upper Materials of Fujian Province (Fujian Huafeng New Material Co., Ltd.), Putian, 351144, China;

  • e PetroChina Petrochemical Research Institute, Beijing, 102206, China

Funds:

21978246), the National Key Research and Development Program of China (Grant No. 2019YFB1503903), the Key Area Research and Development Program of Guangdong Province (Grant No. 2020B0101070001), the Fundamental Research Funds for the Central Universities (Grant No. 20720190014), PetroChina Innovation Foundation (2019D-5007-0413).

We are grateful for funding supported by the National Natural Science Foundation of China (Grant Nos. 22078275

  • Received date 26 July 2021, Accepted date 25 October 2021, RevRecd date 23 September 2021, Publish date 24 November 2021,
    Abstract
  • The selective oxidation of 5-hydroxymethylfurfural (HMF), a versatile bio-based platform molecule, leads to the formation of several intriguing and useful downstream chemicals, such as 2,5-diformylfuran (DFF), 5-hydroxymethyl-2-furancarboxylic acid (HMFCA), formyl 2-furancarboxylic acid (FFCA), 2,5-furandicarboxylic acid (FDCA) and furan-2,5-dimethylcarboxylate (FDMC). These products have been extensively employed to fabricate novel polymers, pharmaceuticals, sustainable dyes and many other value-added fine chemicals. The heart of the developed HMF oxidation processes is always the catalyst. In this regard, this review comprehensively summarized the established heterogeneous catalyst design strategy for the selective oxidation of HMF via thermo-catalysis. Particular attention has been focused on the reaction mechanism of HMF oxidation over different catalysts as well as enhancing the catalytic performance of the catalyst through manipulating the properties of the support and fabricating of multi-component metal nano-particles and oxides. The current challenges and possible research directions for the catalytic oxidation of HMF in the future are also discussed.

     

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