Volume 7 Issue 5
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Xinyu Luo, Wenchao Peng, Yang Li, Fengbao Zhang, Xiaobin Fan. Understanding of the electrochemical behaviors of aqueous zinc–manganese batteries: Reaction processes and failure mechanisms. Green Energy&Environment, 2022, 7(5): 858-899. doi: 10.1016/j.gee.2021.08.006
Citation: Xinyu Luo, Wenchao Peng, Yang Li, Fengbao Zhang, Xiaobin Fan. Understanding of the electrochemical behaviors of aqueous zinc–manganese batteries: Reaction processes and failure mechanisms. Green Energy&Environment, 2022, 7(5): 858-899. doi: 10.1016/j.gee.2021.08.006
shu

Understanding of the electrochemical behaviors of aqueous zinc–manganese batteries: Reaction processes and failure mechanisms

doi: 10.1016/j.gee.2021.08.006

  • a School of Chemical Engineering and Technology, State Key Laboratory of Chemical Engineering, Collaborative Innovation Center of Chemical Science and Engineering, Tianjin University, Tianjin, 300072, China;

  • b Chemistry and Chemical Engineering Guangdong Laboratory, Shantou, 515031, China

Funds:

This study is supported by the National Natural Science Foundation of China (No. 21878226, No. U20A20153), the Chemistry and Chemical Engineering Guangdong Laboratory (Grant No. 1912011) and is dedicated to the 100th anniversary of Chemistry at Nankai University.

  • Received date 23 June 2021, Accepted date 31 August 2021, RevRecd date 29 July 2021, Publish date 01 September 2021,
    Abstract
  • As one of the most common cathode materials for aqueous zinc-ion batteries (AZIBs), manganese oxides have the advantages of abundant reserves, low cost, and low toxicity. However, the electrochemical mechanism at the cathode of aqueous zinc–manganese batteries (AZMBs) is complicated due to different electrode materials, electrolytes and working conditions. These complicated mechanisms severely limit the research progress of AZMBs system and the design of cells with better performance. Hence, the mechanism of AZMBs currently recognized by most researchers according to the classification of the main ions involved in the faradaic reaction is introduced in the review. Then a series of reasons that affect the electrochemical behavior of the battery are summarized. Finally, the failure mechanisms of AZMBs over prolonged cycling are discussed, and the current insufficient research areas of the system are explained, along with the direction of further research being prospected.

     

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