Volume 7 Issue 2
Apr.  2022
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Hao Wan, Wei Ma, Kechao Zhou, Yijun Cao, Xiaohe Liu, Renzhi Ma. Advanced silicon nanostructures derived from natural silicate minerals for energy storage and conversion. Green Energy&Environment, 2022, 7(2): 205-220. doi: 10.1016/j.gee.2021.04.001
Citation: Hao Wan, Wei Ma, Kechao Zhou, Yijun Cao, Xiaohe Liu, Renzhi Ma. Advanced silicon nanostructures derived from natural silicate minerals for energy storage and conversion. Green Energy&Environment, 2022, 7(2): 205-220. doi: 10.1016/j.gee.2021.04.001
shu

Advanced silicon nanostructures derived from natural silicate minerals for energy storage and conversion

doi: 10.1016/j.gee.2021.04.001

  • a School of Chemical Engineering, Zhengzhou University, Zhengzhou, 450001, China;

  • b State Key Laboratory of Powder Metallurgy, Central South University, Changsha, 410083, China;

  • c International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science (NIMS), Namiki 1-1, Tsukuba, Ibaraki, 305-0044, Japan

Funds:

This work is financially supported by National Natural Science Foundation of China (51702291, 51874357, U20A20123), the China Postdoctoral Science Foundation (2020M682352), and State Key Laboratory of Powder Metallurgy, Central South University, Changsha, China. H. W. acknowledges support from the Youth Talent Program of Zhengzhou University and Henan Provincial Key Technology R&D Program (212102210597).

  • Received date 22 January 2021, Accepted date 02 April 2021, RevRecd date 21 March 2021, Publish date 06 April 2021,
    Abstract
  • To effectively alleviate the ever-increasing energy crisis and environmental issues, clean and sustainable energy-related materials as well as the corresponding storage/conversion devices are in urgent demand. Silicon (Si) with the second most elemental abundance on the crust in the form of silicate or silica (SiO2) minerals, is an advanced emerging material showing high performance in energy-related fields (e.g. batteries, photocatalytic hydrogen evolution). For the improved performance in industry-scale applications, Si materials with delicate nanostructures and ideal compositions in a massive production are highly cherished. On account of the reserve, low cost and diverse micro-nanostructures, silicate minerals are proposed as promising raw materials. In the article, crystal structures and the reduction approaches for silicate minerals, as well as recent progress on the as-reduced Si products for clean energy storage/conversion, are presented systematically. Moreover, some cutting-edge fields involving Si materials are discussed, which may offer deep insights into the rational design of advanced Si nanostructures for extended energy-related fields.

     

    • • Si nanomaterials of diverse morphologies extracted from natural silicate minerals were reviewed for the first time. • Both energy storage/conversion applications of Si nanostructures prepared via the reduction strategies were summarized. • Several typical reduction strategies for the thermic reduction of natural silicate minerals were introduced.
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