Volume 7 Issue 6
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Xiaoying Guo, Xusheng Zhang, Yingxiong Wang, Xiaodong Tian, Yan Qiao. Converting furfural residue wastes to carbon materials for high performance supercapacitor. Green Energy&Environment, 2022, 7(6): 1270-1280. doi: 10.1016/j.gee.2021.01.021
Citation: Xiaoying Guo, Xusheng Zhang, Yingxiong Wang, Xiaodong Tian, Yan Qiao. Converting furfural residue wastes to carbon materials for high performance supercapacitor. Green Energy&Environment, 2022, 7(6): 1270-1280. doi: 10.1016/j.gee.2021.01.021
shu

Converting furfural residue wastes to carbon materials for high performance supercapacitor

doi: 10.1016/j.gee.2021.01.021

  • a. State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan, 030001, China;

  • b. Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049, China;

  • c. CAS Key Laboratory of Carbon Materials, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan, 030001, China;

  • d. Shanxi Engineering Research Center of Biorefinery, Institute of Coal Chemistry, Chinese Academy of Sciences, 27 South Taoyuan Road, Taiyuan, 030001, China

Funds:

This work was financially supported by the National Natural Science Foundation of China (22075308, U1710106, U1810111), Natural Science Foundation of Shanxi Province (No: 201801D221371) and Shanxi Province Science Foundation for Youths (No: SQ2019001).

  • Received date 25 November 2020, Accepted date 29 January 2021, RevRecd date 29 January 2021, Publish date 31 December 2022,
    Abstract
  • Sustainable development based on the value-added utilization of furfural residues (FRs) is an effective way to achieve a profitable circular economy. This comprehensive work highlights the potential of FRs as precursor to prepare porous carbons for high performance supercapacitors (SCs). To improve the electrochemical performance of FR-based carbon materials, a facile route based on methanol pretreatment coupled with pre-carbonization and followed KOH activation is proposed. More defects could be obtained after methanol treatment, which is incline to optimize textural structure. The activated methanol treated FR-based carbon materials (AFRMs) possess high specific surface area (1753.5 m2 g-1), large pore volume (0.85 cm3 g-1), interconnected micro/mesoporous structure, which endow the AFRMs with good electrochemical performance in half-cell (326.1 F g-1 at 0.1 A g-1, 189.4 F g-1 at 50 A g-1 in 6 mol L-1 KOH). The constructed symmetric SCs based on KOH, KOH–K3Fe(CN)6 and KOH-KI electrolyte deliver energy density up to 8.9, 9.9 and 10.6 Wh kg-1 with a capacitance retention of over 86% after 10,000 cycles. Furthermore, the self-discharge can be restrained by the addition of K3Fe(CN)6 and KI in KOH electrolyte. This study provides an effective approach for high-valued utilization of FR waste.

     

    • • The application of furfural residue wastes in energy storage device is proposed. • Facile route of methanol treatment is favorable to optimize pore size distribution. • As-obtained activated carbon exhibits good performance in different electrolytes. • The device assembled by redox electrolyte shows boosted energy density and retention.
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