Volume 7 Issue 5
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Article Navigation >  Green Energy&Environment  > 2022  >  7(5): 1053-1061
Yuchen Wang, Zuo Chen, Man Zhang, Yaoyu Liu, Huixia Luo, Kai Yan. Green fabrication of nickel-iron layered double hydroxides nanosheets efficient for the enhanced capacitive performance. Green Energy&Environment, 2022, 7(5): 1053-1061. doi: 10.1016/j.gee.2021.01.019
Citation: Yuchen Wang, Zuo Chen, Man Zhang, Yaoyu Liu, Huixia Luo, Kai Yan. Green fabrication of nickel-iron layered double hydroxides nanosheets efficient for the enhanced capacitive performance. Green Energy&Environment, 2022, 7(5): 1053-1061. doi: 10.1016/j.gee.2021.01.019
shu

Green fabrication of nickel-iron layered double hydroxides nanosheets efficient for the enhanced capacitive performance

doi: 10.1016/j.gee.2021.01.019

  • a School of Environmental Science and Engineering, Sun Yat-sen University, 135 Xingang Xi Road, Guangzhou, 510275, China;

  • b Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology, Guangzhou, 510275, China;

  • c Key Lab of Polymer Composite & Functional Materials, School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou, 510275, China

Funds:

The authors acknowledged the financial supports from Key-Area Research and Development Program of Guangdong Province (2019B110209003), Guangdong Basic and Applied Basic Research Foundation (2019B1515120058, 2020A1515011149), National Key R&

D Program of China (2018YFD0800700), National Ten Thousand Talent Plan, National Natural Science Foundation of China (21776324), the Fundamental Research Funds for the Central Universities (19lgzd25), and Hundred Talent Plan (201602) from Sun Yat-sen University.

  • Received date 28 October 2020, Accepted date 21 January 2021, RevRecd date 21 January 2021, Publish date 23 January 2021,
    Abstract
  • Rational synthesis of robust layered double hydroxides (LDHs) nanosheets for high-energy supercapacitors is full of challenges. Herein, we reported an ultrasonication-assisted strategy to eco-friendly fabricate NiFe-LDHs nanosheets for the enhanced capacitive behavior. The experimental results combined with different advanced characterization tools document that the utilization of ultrasonication has a profound effect on the morphology and thickness of the as-obtained NiFe-LDHs, alternatively affecting the capacitive behavior. It shows that NiFe-LDHs nanosheets prepared with 2-h ultrasonic treatments display the exceptional capacitive performance because of the synergetic effect of ultrathin thickness, large specific surface area, and high mesoporous volume. The maximum specific capacitance of Ni3Fe1-LDHs nanosheets with the thickness of 7.39 nm and the specific surface area of 77.16 m2 g-1 reached 1923 F g-1, which is competitive with most previously reported values. In addition, the maximum specific energy of the assembled NiFe-LDHs//AC asymmetric supercapacitor achieved 49.13 Wh kg-1 at 400 W kg-1. This work provides a green technology to fabricate LDHs nanosheets, and offers deep insights for understanding the relationship between the morphology/structure and capacitive behavior of LDHs nanosheets, which is helpful for achieving high-performance LDHs-based electrode materials.

     

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