Volume 7 Issue 1
Feb.  2022
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Qixing Du, Yanmei Gong, Muhammad Arif Khan, Daixin Ye, Jianhui Fang, Hongbin Zhao, Jiujun Zhang. Regulating non-precious transition metal nitrides bifunctional electrocatalysts through surface/interface nanoengineering for air-cathodes of Zn-air batteries. Green Energy&Environment, 2022, 7(1): 16-34. doi: 10.1016/j.gee.2021.01.018
Citation: Qixing Du, Yanmei Gong, Muhammad Arif Khan, Daixin Ye, Jianhui Fang, Hongbin Zhao, Jiujun Zhang. Regulating non-precious transition metal nitrides bifunctional electrocatalysts through surface/interface nanoengineering for air-cathodes of Zn-air batteries. Green Energy&Environment, 2022, 7(1): 16-34. doi: 10.1016/j.gee.2021.01.018
shu

Regulating non-precious transition metal nitrides bifunctional electrocatalysts through surface/interface nanoengineering for air-cathodes of Zn-air batteries

doi: 10.1016/j.gee.2021.01.018

  • a Department of Chemistry & Institute for Sustainable Energy, College of Sciences, Shanghai University, Shanghai, 200444, China;

  • b Department of Physics, College of Sciences, Shanghai University, Shanghai, 200444, China;

  • c School of Material Science and Engineering, Shanghai University, Shanghai, 200444, China

  • Received date 21 November 2020, Accepted date 20 January 2021, RevRecd date 31 December 2020, Publish date 23 January 2021,
    Abstract
  • Zn-air batteries (ZABs), especially the secondary batteries, have engrossed a great interest because of its high specific energy, economical and high safety. However, due to the insufficient activity and stability of bifunctional electrocatalysts for air-cathode oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) processes, the practical application of rechargeable ZABs is seriously hindered. In the effort of developing high active, stable and cost-effective electrocatalysts, transition metal nitrides (TMNs) have been regarded as the candidates due to their high conductivity, strong corrosion-resistance, and bifunctional catalytic performance. In this paper, the research progress in TMNs-based material as ORR and OER electrocatalysts for ZABs is discussed with respect to their synthesis, chemical/physical characterization, and performance validation/optimization. The surface/interface nanoengineering strategies such as defect engineering, support binding, heteroatom introduction, crystal plane orientation, interface construction and small size effect, the physical and chemical properties of TMNs-based electrocatalysts are emphasized with respect to their structures/morphologies, composition, electrical conductivity, specific surface area, chemical stability and corrosion resistance. The challenges of TMNs-based materials as bifunctional air-cathode electrocatalysts in practical application are evaluated, and numerous research guidelines to solve these problems are put forward for facilitating further research and development.

     

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