Volume 7 Issue 5
Oct.  2022
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Shuai Cao, Jingyun Jiang, Qingyong Tian, Cang Guo, Xuzhe Wang, Kun Dai, Qun Xu. Building of multifunctional and hierarchical HxMoO3/PNIPAM hydrogel for high-efficiency solar vapor generation. Green Energy&Environment, 2022, 7(5): 1006-1013. doi: 10.1016/j.gee.2020.12.012
Citation: Shuai Cao, Jingyun Jiang, Qingyong Tian, Cang Guo, Xuzhe Wang, Kun Dai, Qun Xu. Building of multifunctional and hierarchical HxMoO3/PNIPAM hydrogel for high-efficiency solar vapor generation. Green Energy&Environment, 2022, 7(5): 1006-1013. doi: 10.1016/j.gee.2020.12.012

Building of multifunctional and hierarchical HxMoO3/PNIPAM hydrogel for high-efficiency solar vapor generation

doi: 10.1016/j.gee.2020.12.012
  • Solar distillation is a sustainable and promising technique to generate fresh water. However, the solar vapor generation is a high energy consumption process, resulting in a low water yield under natural sunlight. Hence, developing of advanced evaporators that can simultaneously reduce the energy requirement of water vaporization and accelerate solar water evaporation remains a great challenge. In this study, we report the fabrication of a multifunctional hydrogel of HxMoO3/PNIPAM with PNIPAM as hydratable skeleton and HxMoO3 as the light-absorbing unit for solar water evaporation. The experimental results demonstrate that the as-prepared hydrogel owns excellent photothermal activity. Accurately, the fabricated hydrogel -based solar evaporators achieved high water evaporation rate of 1.65 kg m-2 h-1 with the energy conversion efficiency of 85.87% under 1 kW m-2 irradiation. The enhanced photothermal activity of HxMoO3/PNIPAM hydrogel can be attributed to the synergistic effects of the components composed in this hierarchical architecture that change the water state and further speed up water evaporation. The HxMoO3/PNIPAM evaporators indicate its great potential for practical implementation of solar water evaporation.

     

  • These authors contributed equally.
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  • [1]
    Y. Guo, J. Bae, Z. Fang, P. Li, F. Zhao, G. Yu, Chem. Rev. 120 (2020) 7642-7707
    [2]
    H. Liu, Z. Huang, K. Liu, X. Hu, J. Zhou, Adv. Energy Mater. 9 (2019) 1900310
    [3]
    C. Chen, Y. Kuang, L. Hu, Joule 3 (2019) 683-718
    [4]
    Z. Wang, T. Horseman, A.P. Straub, N.Y. Yip, D. Li, M. Elimelech, S. Lin, Sci. Adv. 5 (2019) eaax0763
    [5]
    N. Xu, J. Li, Y. Wang, C. Fang, X. Li, Y. Wang, L. Zhou, B. Zhu, Z. Wu, S. Zhu, J. Zhu, Sci. Adv. 5 (2019) eaaw7013
    [6]
    X. Zhou, Y. Guo, F. Zhao, G. Yu, Acc. Chem. Res. 52 (2019) 3244-3253
    [7]
    Q. Ma, P. Yin, M. Zhao, Z. Luo, Y. Huang, Q. He, Y. Yu, Z. Liu, Z. Hu, B. Chen, H. Zhang, Adv. Mater. 31 (2019) e1808249
    [8]
    P. Tao, G. Ni, C. Song, W. Shang, J. Wu, J. Zhu, G. Chen, T. Deng, Nat. Energy 3 (2018) 1031-1041
    [9]
    F. Zhao, Y. H. Guo, X.Y. Zhou, W. Shi, G. H. Yu, Nat. Rev. Mater. 5 (2020) 388-401
    [10]
    F. Yu, X. Ming, Y. Xu, Z. Chen, D. Meng, H. Cheng, Z. Shi, P. Shen, X. Wang, Adv. Mater. Interfaces 6 (2019) 1901168
    [11]
    W. Huang, P. Su, Y. Cao, C. Li, D. Chen, X. Tian, Y. Su, B. Qiao, J. Tu, X. Wang, Nano Energy 69 (2020) 104465
    [12]
    Z. Sun, J. Wang, Q. Wu, Z. Wang, Z. Wang, J. Sun, C.J. Liu, Adv. Funct. Mater. 29 (2019) 1901312
    [13]
    L. Zhou, Y. Tan, D. Ji, B. Zhu, P. Zhang, J. Xu, Q. Gan, Z. Yu, J. Zhu, Sci. Adv. 2 (2016) e1501227
    [14]
    X. Zhou, Y. Guo, Y. Zhang, G. H. Yu, Energy Environ. Sci. 11 (2018) 1985-1992
    [15]
    F. Wang, D. Wei, Y. Li, T. Chen, P. Mu, H. Sun, Z. Zhu, W. Liang, A. Li, J. Mater. Chem. A 7 (2019) 18311-18317
    [16]
    L. Wu, Z. Dong, Z. Cai, T. Ganapathy, N. X. Fang, C. Li, C. Yu, Y. Zhang, Y. Song, Nat. Commun. 11 (2020) 521
    [17]
    P. Zhang, F. Liu, Q. Liao, H. Yao, H. Geng, H. Cheng, C. Li, L. Qu, Angew. Chem. Int. Ed. 57 (2018) 16343-16347
    [18]
    F. Zhao, X. Zhou, Y. Liu, Y. Shi, Y. Dai, G. Yu, Adv. Mater. 31 (2019) e1806446
    [19]
    H. Geng, Q. Xu, M. Wu, H. Ma, P. Zhang, T. Gao, L. Qu, T. Ma, C. Li, Nat. Commun. 10 (2019) 1512
    [20]
    X. Zhou, F. Zhao, Y. Guo, B. Rosenberger, G. H. Yu, Sci. Adv. 5 (2019) eaaw5484
    [21]
    C. Y. Song, B. Y. Zhang, L. Hao, J. K. Min, N. Liu, R. Niu, J. Gong, T. Tang, Green Energy & Environment (2020), https://doi.org/10.1016/j.gee.2020.10.002
    [22]
    W. Xu, X. Hu, S. Zhuang, Y. Wang, X. Li, L. Zhou, S. Zhu, J. Zhu, Adv. Energy Mater. 8 (2018) 1702884
    [23]
    F. Zhao, X. Zhou, Y. Shi, X. Qian, M. Alexander, X. Zhao, S. Mendez, R. Yang, L. Qu, G. H. Yu, Nat. Nanotechnol. 13 (2018) 489-495
    [24]
    H. B. Xu, K. L. Yu, M. Y. Pan, Z. P. Yao, T. Q. Zhao, Z. H. Jiang, Green Energy & Environment (2020), https://doi.org/10.1016/j.gee.2020.10.010
    [25]
    S. Zhang, Y. Chen, H. Liu, Z. Wang, H. Ling, C. Wang, J. Ni, B. Celebi-Saltik, X. Wang, X. Meng, H.J. Kim, A. Baidya, S. Ahadian, N. Ashammakhi, M. R. Dokmeci, J. Travas-Sejdic, A. Khademhosseini, Adv. Mater. 32 (2020) e1904752
    [26]
    Y. S. Zhang, A. Khademhosseini, Science 356 (2017) eaaf3627
    [27]
    Y. Guo, X. Zhou, F. Zhao, J. Bae, B. Rosenberger, G. H. Yu, ACS Nano 13 (2019) 7913-7919
    [28]
    X. Wang, P. Yan, Q. Xu, H. Li, C. Guo, C. Liu, Chem. Commun. 55 (2019) 9777-9780
    [29]
    C. Guo, P. Yan, C. Zhu, C. Wei, W. Liu, W. Wu, X. Wang, L. Zheng, J. Wang, Y. Du, J. Chen, Q. Xu, Chem. Commun. 55 (2019) 12527-12530
    [30]
    W. Liu, Q. Xu, W. Cui, C. H. Zhu, Y.H Qi, Angew. Chem. Int. Ed. 56 (2017) 1-6
    [31]
    H. Li, Q. Xu, X. Wang, W. Liu, Small 14 (2018) e1801523
    [32]
    T. Hirata, K. Ishioka, M. Kitajima, Appl. Phys. Lett. 68 (1996) 458-460
    [33]
    J. Song, X. Ni, L. Gao, H. Zheng, Mater. Chem. Phys. 102 (2007) 245-248
    [34]
    S. Adams, J. Solid State Chem. 149 (2000) 75-87
    [35]
    X. Tong, L.N. Du, Q. Xu, J. Mater Chem A 6 (2018) 3091-3099
    [36]
    S. Cao, X. Tong, K. Dai, Q. Xu, J. Mater Chem A 7 (2019) 8204-8209
    [37]
    Y. Katsumoto, H. Komatsu, K. Ohno, J. Am. Chem. Soc. 128 (2006) 9278-9279
    [38]
    B. J. van der Veken, R. Szostak, D. N. Shchepkin, Z. Havlas, P. Hobza, J. Am. Chem. Soc. 123 (2001) 12290-12293
    [39]
    C. Yan, P. L. Kramer, R. Yuan, M. D. Fayer, J. Am. Chem. Soc. 140 (2018) 9466-9477
    [40]
    T. Baba, R. Sakamoto, M. Shibukawa, K. Oguma, J. Chromatogr. A 1040 (2004) 45-51
    [41]
    Y. Sekine, T. Ikeda-Fukazawa, J. Chem. Phys. 130 (2009) 034501
    [42]
    A. Eklund, H. Zhang, H. Zeng, A. Priimagi, O. Ikkala, Adv. Funct. Mater. 30 (2020) 2000754
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