Volume 7 Issue 4
Aug.  2022
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Article Navigation >  Green Energy&Environment  > 2022  >  7(4): 818-828
Changde Ma, Jiang Gong, Shuang Zhao, Xiaoguang Liu, Xueying Mu, Yanhui Wang, Xuecheng Chen, Tao Tang. One-pot green mass production of hierarchically porous carbon via a recyclable salt-templating strategy. Green Energy&Environment, 2022, 7(4): 818-828. doi: 10.1016/j.gee.2020.12.004
Citation: Changde Ma, Jiang Gong, Shuang Zhao, Xiaoguang Liu, Xueying Mu, Yanhui Wang, Xuecheng Chen, Tao Tang. One-pot green mass production of hierarchically porous carbon via a recyclable salt-templating strategy. Green Energy&Environment, 2022, 7(4): 818-828. doi: 10.1016/j.gee.2020.12.004
shu

One-pot green mass production of hierarchically porous carbon via a recyclable salt-templating strategy

doi: 10.1016/j.gee.2020.12.004

  • a State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun, 130022, China;

  • b University of Science and Technology of China, Hefei, 230026, China;

  • c Key Laboratory for Material Chemistry of Energy Conversion and Storage, Ministry of Education, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, China;

  • d Faculty of Chemical Technology and Engineering, West Pomeranian University of Technology, Piastów Ave42, Szczecin, 71-065, Poland

Funds:

This work is supported by the National Natural Science Foundation of China (No. 51303170), and the National Science Centre, Poland within BEETHOVEN UMO-2016/23/G/ST5/04200.

  • Received date 16 July 2020, Accepted date 06 December 2020, RevRecd date 29 October 2020, Publish date 10 December 2020,
    Abstract
  • Porous carbon materials have exhibited a series of promising applications in supercapacitors and other research fields, yet still confronting the complicated synthetic procedures and massive usage of toxic reagents. Herein, we propose a green and one-pot method to produce heteroatom-doped hierarchical porous carbon materials in large-scale without any toxic reagents employed. Eventually, the as-prepared nitrogen-doped porous carbon (NPC) displays a high specific surface area of 2018 m2 g-1 together with abundant heteroatom dopants (14.8 wt% O and 1.03 wt% N). The potassium carbonate template can be recycled via a simple rinsing and re-precipitation process. Furthermore, the as-prepared nitrogen-doped porous carbon delivers a high specific capacitance of 361 F g-1 at 0.5 A g-1 and excellent rate capability of 240 F g-1 at 20 A g-1 (66.5% capacitance retention). Finally, considering the low-price raw materials and facile green synthesis procedure, the present approach can be easily scalable to prepare biomass-derived heteroatoms doped porous carbon, which is not only applicable for supercapacitor but also for other research fields.

     

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