Volume 6 Issue 3
Jun.  2021
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Article Navigation >  Green Energy&Environment  > 2021  >  6(3): 314-328
Yanrong Liu, Zhengxing Dai, Zhibo Zhang, Shaojuan Zeng, Fangfang Li, Xiangping Zhang, Yi Nie, Lei Zhang, Suojiang Zhang, Xiaoyan Ji. Ionic liquids/deep eutectic solvents for CO2 capture: Reviewing and evaluating. Green Energy&Environment, 2021, 6(3): 314-328. doi: 10.1016/j.gee.2020.11.024
Citation: Yanrong Liu, Zhengxing Dai, Zhibo Zhang, Shaojuan Zeng, Fangfang Li, Xiangping Zhang, Yi Nie, Lei Zhang, Suojiang Zhang, Xiaoyan Ji. Ionic liquids/deep eutectic solvents for CO2 capture: Reviewing and evaluating. Green Energy&Environment, 2021, 6(3): 314-328. doi: 10.1016/j.gee.2020.11.024
shu

Ionic liquids/deep eutectic solvents for CO2 capture: Reviewing and evaluating

doi: 10.1016/j.gee.2020.11.024
  • a.

    Energy Engineering, Division of Energy Science, Luleå University of Technology, Luleå, Sweden

  • b.

    Swerim AB, Box 812, SE-97125, Luleå, Sweden

  • c.

    State Key Laboratory of Material-Oriented Chemical Engineering, Nanjing Tech University, Nanjing, China

  • d.

    CAS Key Laboratory of Green Process and Engineering, Beijing Key Laboratory of Ionic Liquids Clean Process, State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences, Beijing, China

  • e.

    Zhengzhou Institute of Emerging Industrial Technology, Zhengzhou, China

  • f.

    College of Materials Science and Engineering, Fujian University of Technology, Fuzhou, Fujian, 350118, China

  • g.

    School of Chemical Engineering, University of Chinese Academy of Sciences, Beijing, China

More Information
  • Corresponding author: E-mail address: sjzhang@ipe.ac.cn (Suojiang Zhang); E-mail address: xiaoyan.ji@ltu.se (Xiaoyan Ji)
  • Received date 30 August 2020, Accepted date 24 November 2020, Available online 28 November 2020, Publish date 30 June 2021,
    Abstract

  • The CO2 solubilities (including CO2 Henry's constant) in physical- and chemical-based ILs/DESs and the COSMO-RS models describing these properties were comprehensively collected and summarized. The summarized results indicate that chemical-based ILs/DESs are superior to physical-based ILs/DESs for CO2 capture, especially those ILs have functionalized cation and anion, and superbase DESs; some of the superbase DESs have higher CO 2 solubilities than those of ILs; the best physical- and chemical-based ILs, as well as physical- and chemical-based DESs are [BMIM][BF4] (4.20 mol kg−1), [DETAH][Im] (11.91 mol kg−1), [L-Arg]-Gly 1:6 (4.92 mol kg−1) and TBD-EG 1:4 (12.90 mol kg−1), respectively. Besides the original COSMO-RS mainly providing qualitative predictions, six corrected COSMO-RS models have been proposed to improve the prediction performance based on the experimental data, but only one model is with universal parameters. The newly determined experimental results were further used to verify the perditions of original and corrected COSMO-RS models. The comparison indicates that the original COSMO-RS qualitatively predicts CO2 solubility for some but not all ILs/DESs, while the quantitative prediction is incapable at all. The original COSMO-RS is capable to predict CO2 Henry's constant qualitatively for both physical-based ILs and DESs, and quantitative prediction is only available for DESs. For the corrected COSMO-RS models, only the model with universal parameters provides quantitative predictions for CO2 solubility in physical-based DESs, while other corrected models always show large deviations (> 83%) compared with the experimental CO2 Henry's constants.

     

    The CO2 solubility (including Henry's constant) in ILs/DESs and the COSMO-RS models describing these properties were collected, and compared with the original and corrected COSMO-RS prediction results. Then the best CO2 solubility and the performance of COSMO-RS models were achieved.

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