Volume 7 Issue 3
Jun.  2022
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Article Navigation >  Green Energy&Environment  > 2022  >  7(3): 423-431
Gaopeng Liu, Bin Wang, Lin Wang, Wenxian Wei, Yu Quan, Chongtai Wang, Wenshuai Zhu, Huaming Li, Jiexiang Xia. MOFs derived FeNi3 nanoparticles decorated hollow N-doped carbon rod for high-performance oxygen evolution reaction. Green Energy&Environment, 2022, 7(3): 423-431. doi: 10.1016/j.gee.2020.10.007
Citation: Gaopeng Liu, Bin Wang, Lin Wang, Wenxian Wei, Yu Quan, Chongtai Wang, Wenshuai Zhu, Huaming Li, Jiexiang Xia. MOFs derived FeNi3 nanoparticles decorated hollow N-doped carbon rod for high-performance oxygen evolution reaction. Green Energy&Environment, 2022, 7(3): 423-431. doi: 10.1016/j.gee.2020.10.007
shu

MOFs derived FeNi3 nanoparticles decorated hollow N-doped carbon rod for high-performance oxygen evolution reaction

doi: 10.1016/j.gee.2020.10.007

  • a School of Chemistry and Chemical Engineering, Institute for Energy Research, Jiangsu University, 301 Xuefu Road, Zhenjiang, 212013, China;

  • b Testing Center, Yangzhou University, Yangzhou, Jiangsu, 225009, China;

  • c School of Chemistry and Chemical Engineering, The Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Hainan Normal University, Haikou, Hainan, 571158, China

Funds:

This work was financially supported by the National Natural Science Foundation of China (Nos. 21576123 and 21878134), and Jiangsu University Scientific Research Funding (No. 11JDG0146).

  • Received date 29 June 2020, Accepted date 10 October 2020, RevRecd date 16 September 2020, Publish date 14 October 2020,
    Abstract
  • The sluggish electrochemical oxygen evolution reaction (OER) is a crucial process for clean energy conversion technology. The preparation of non-precious electrocatalysts with high performance for OER is still a main challenge. Herein, we report a FeNi3 nanoparticles incorporated on N-doped hollow carbon rod with extraordinary performance toward OER by in situ annealing the Ni-doped Fe based metal-organic frameworks (MOFs) precursors. Meanwhile, the pristine N atoms of MOFs doped into carbon frameworks can enhance the electrical conductivity, boost electron mass transport and electron transfer, and construct more active sites. Furthermore, constructing the Fe-Ni alloy structure can facilitate the formation of O-O bond, optimize the free energy for intermediate adsorption and improve OER performance. The as-prepared Fe-Ni bimetal decorated hollow N-doped nanocarbon hybrid structure possesses superior OER performance, which is surpass commercial IrO2 at a overpotential of only 340 mV to achieve the current density of 10 mA cm−2, as well as a small Tafel slope of 86.67 mV dec−1 in alkaline electrolyte. The Fe-Ni alloy/hollow N-doped nanocarbon hybrid structure shining the bright future for obtaining earth-abundant and superior efficient anode OER electrocatalyst.

     

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