Volume 7 Issue 2
Apr.  2022
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Article Navigation >  Green Energy&Environment  > 2022  >  7(2): 229-235
Yanxue Guo, Hui Liu, Dong Chen, Jianglan Qu, Jun Yang. High recycling Fe3O4-CdTe nanocomposites for the detection of organophosphorothioate pesticide chlorpyrifos. Green Energy&Environment, 2022, 7(2): 229-235. doi: 10.1016/j.gee.2020.09.001
Citation: Yanxue Guo, Hui Liu, Dong Chen, Jianglan Qu, Jun Yang. High recycling Fe3O4-CdTe nanocomposites for the detection of organophosphorothioate pesticide chlorpyrifos. Green Energy&Environment, 2022, 7(2): 229-235. doi: 10.1016/j.gee.2020.09.001
shu

High recycling Fe3O4-CdTe nanocomposites for the detection of organophosphorothioate pesticide chlorpyrifos

doi: 10.1016/j.gee.2020.09.001

  • a Department of Applied Chemistry, Key Laboratory of Urban Agriculture (North China), Ministry of Agriculture and Rural Affairs, Beijing University of Agriculture, Beijing, 102206, China;

  • b State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences, Beijing, 100190, China;

  • c University of Chinese Academy of Sciences, No. 19A Yuquan Road, Beijing, 100049, China;

  • d Zhongke Langfang Institute of Process Engineering, Fenghua Road No 1, Langfang Economic & Technical Development Zone, Hebei Province, 065001, China

Funds:

This work was supported by the Importation and Development of High-Caliber Talents Project of Beijing Municipal Institutions (CIT&TCD201704049), the Development of Beijing Excellent Talents Project (2016000026833ZK01), Beijing Municipal Natural Science Foundation (2202015), the Technology Innovation Project of Beijing Municipal Institutions (KM201610020001), the National Natural Science Foundation of China (21706265), and State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences (MPCS-2019-A-09).

  • Received date 13 May 2020, Accepted date 10 September 2020, RevRecd date 09 September 2020, Publish date 12 September 2020,
    Abstract
  • To alleviate the secondary contamination of our environment when using quantum dots (QDs) to detect the organophosphorothioate pesticides (OPPs), we herein report a strategy to assemble magnetic Fe3O4 nanoparticles and luminescent CdTe quantum dots (QDs) into a composite nanosystem, which possesses both the magnetic property of Fe3O4 nanoparticles and the luminescent character of CdTe QDs, for the detection of chlorpyrifos, one of the typical OPPs. This strategy involves the isolated synthesis of magnetic Fe3O4 nanoparticles with positive charges and luminescent CdTe QDs with negative charges, and their subsequent assembly by electrostatic interaction. The as-prepared Fe3O4–CdTe nanocomposites have a detection limit as low as 10 ppb for chlorpyrifos, and are also selective for the OPPs with a phosphorothioate moiety (P＝S bond). In specific, the Fe3O4–CdTe nanocomposites can be conveniently harvested by a normal magnet, and the recycling rate for both Cd and Fe determined by inductively coupled plasma atomic emission spectroscopy (ICP-AES) is higher than 96%, showing great potential in alleviating the Cd pollution on the environment.

     

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