Volume 7 Issue 1
Feb.  2022
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Article Navigation >  Green Energy&Environment  > 2022  >  7(1): 75-85
Zunhang Lv, Kaihang Wang, Yingying Si, Zihan Li, Tianpeng Yu, Xin Liu, Guixue Wang, Guangwen Xie, Luhua Jiang. High performance of multi-layered alternating Ni-Fe-P and Co-P films for hydrogen evolution. Green Energy&Environment, 2022, 7(1): 75-85. doi: 10.1016/j.gee.2020.07.023
Citation: Zunhang Lv, Kaihang Wang, Yingying Si, Zihan Li, Tianpeng Yu, Xin Liu, Guixue Wang, Guangwen Xie, Luhua Jiang. High performance of multi-layered alternating Ni-Fe-P and Co-P films for hydrogen evolution. Green Energy&Environment, 2022, 7(1): 75-85. doi: 10.1016/j.gee.2020.07.023
shu

High performance of multi-layered alternating Ni-Fe-P and Co-P films for hydrogen evolution

doi: 10.1016/j.gee.2020.07.023

  • College of Materials Science and Engineering, Qingdao University of Science and Technology, No.53 Zhengzhou Road, Qingdao, 266042, China

  • Received date 13 April 2020, Accepted date 26 July 2020, RevRecd date 04 July 2020, Publish date 02 August 2020,
    Abstract
  • Judiciously engineering the electrocatalysts is attractive and challenging to exploit materials with high electrocatalytic performance for hydrogen evolution reaction. Herein, we successfully perform the interface engineering by alternately depositing Co-P and Ni-Fe-P films on nickel foam, via facile electroless plating and de-alloying process. This work shows that there is a significant effect of de-alloying process on alloy growth. The electronic structure of layered alloys is improved by interface engineering. The multilayer strategy significantly promotes the charge transfer. Importantly, the Co-P/Ni-Fe-P/NF electrode fabricated by interface engineering exhibits excellent electrocatalytic hydrogen evolution activity with an overpotential of 43.4 mV at 10 mA cm-2 and long-term durability for 72 h in alkaline medium (1 mol L-1 KOH). The innovative strategy of this work may aid further development of commercial electrocatalysts.

     

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