Volume 7 Issue 1
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Article Navigation >  Green Energy&Environment  > 2022  >  7(1): 53-65
Hong-Li Ding, Hai-Tao Yu, Xiao-dong Wang, Chen-Feng Guo, Bing Zheng, Ying Xie, Ting-Feng Yi. Improving the stability, lithium diffusion dynamics, and specific capacity of SrLi2Ti6O14 via ZrO2 coating. Green Energy&Environment, 2022, 7(1): 53-65. doi: 10.1016/j.gee.2020.07.014
Citation: Hong-Li Ding, Hai-Tao Yu, Xiao-dong Wang, Chen-Feng Guo, Bing Zheng, Ying Xie, Ting-Feng Yi. Improving the stability, lithium diffusion dynamics, and specific capacity of SrLi2Ti6O14 via ZrO2 coating. Green Energy&Environment, 2022, 7(1): 53-65. doi: 10.1016/j.gee.2020.07.014
shu

Improving the stability, lithium diffusion dynamics, and specific capacity of SrLi2Ti6O14 via ZrO2 coating

doi: 10.1016/j.gee.2020.07.014

  • a Key Laboratory of Functional Inorganic Material Chemistry, Ministry of Education, School of Chemistry and Materials Science, Heilongjiang University, Harbin, 150080, China;

  • b College of Material Science and Chemical Engineering, Harbin Engineering University, Harbin, 150001, China;

  • c School of Resources and Materials, Northeastern University at Qinhuangdao, Qinhuangdao, 066004, China;

  • d Institute of Advanced Electrochemical Energy & School of Materials Science and Engineering, Xi'an University of Technology, Xi'an, Shaanxi, 710048, China

  • Received date 31 January 2020, Accepted date 21 July 2020, RevRecd date 17 June 2020, Publish date 26 July 2020,
    Abstract
  • SrLi2Ti6O14 (SLTO) coated with different amount of ZrO2 was successfully prepared. The as-obtained composites are stacked by a series of particles with a pure phase structure and a good crystallinity. Furthermore, ZrO2 coating not only enhances the structural stability of the materials but also facilitates the diffusion of lithium through the SEI film. As a result, the redox polarization was reduced, and the reversibility of the electrochemical reaction was enhanced. Particularly, SLTO-ZrO2-2 sample delivers a high initial lithiation capacity of 283.6 mA h g-1, and the values maintain at 251.7, 228.0, 207.4, 175.3, and 147.7 mA h g-1 at the current densities of 0.13, 0.26, 0.54, 1.31, and 2.62 A g-1, respectively. Our experiment also confirmed that SLTO materials coated with ZrO2 are suitable for high power density applications, and the lithiation specific energy efficiency of SLTO-ZrO2-2 is 200% as high as that of pure SLTO at a power density of 1257 W kg-1.

     

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